Carter Korey P, Pallares Roger M, Abergel Rebecca J
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
Department of Nuclear Engineering, University of California, Berkeley, CA, 94709, USA.
Commun Chem. 2020 Aug 7;3(1):103. doi: 10.1038/s42004-020-00338-5.
Over the past decade, momentous progress has been made in the characterization of late actinide compounds. Here the authors highlight how advances in spectroscopic and computational tools have developed our understanding of fundamental transplutonium bonding interactions, and discuss whether covalency and heterogeneity changes in 5f-orbital bonding could be harnessed in environmentally and industrially relevant systems.
在过去十年里，晚期锕系元素化合物的表征取得了重大进展。在此，作者强调了光谱学和计算工具的进步如何增进了我们对超钚元素基本键合相互作用的理解，并讨论了在与环境和工业相关的体系中，5f轨道键合中的共价性和非均质性变化是否能够得到利用。
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