Impact of interfacial rheology on finger tip splitting.

Fluid-fluid interfaces, laden with polymers, surfactants, lipid bilayers, proteins, solid particles, or other surface-active agents, often exhibit a rheologically complex response to deformations. Despite its academic and practical relevance to fluid dynamics and various other fields of research, the role of interfacial rheology in viscous fingering remains fairly underexplored. A noteworthy exception is the work by Li and Manikantan [Phys. Rev. Fluids 6, 074001 (2021)2469-990X10.1103/PhysRevFluids.6.074001], who used linear stability analysis to show that surface rheological stresses act to stabilize the development of radial viscous fingering at the linear regime. In this paper, we perform a perturbative, second-order mode-coupling analysis of the system and investigate the influence of interfacial rheology on the morphology of the fingering structures at early nonlinear stages of the dynamics. In particular, we focus on understanding how interfacial rheology impacts the emblematic finger tip-widening and finger tip-splitting phenomena that take place in radial viscous fingering in Hele-Shaw cells. We describe the viscous Newtonian fluid-fluid interface by using a Boussinesq-Scriven model, and derive a generalized Young-Laplace pressure jump condition at the fluid-fluid interface. In this framing, we go beyond the purely linear description and use Darcy's law to obtain a perturbative mode-coupling differential equation which describes the time evolution of the perturbation amplitudes, accurate to second order. Our early nonlinear mode-coupling results indicate that regardless of their stabilizing action at the linear regime, interfacial rheology effects favor finger tip widening, leading to the occurrence of enhanced finger tip-splitting events.