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LiF:Mg,Ti(TLD-100)复合峰 5 的热释光(TL)剂量响应:动力学顺序的依赖性。

THE THERMOLUMINESCENCE (TL) DOSE RESPONSE OF COMPOSITE PEAK 5 IN LIF:MG,TI (TLD-100): DEPENDENCE ON THE ORDER OF KINETICS.

机构信息

Physics Unit, Sami Shamoon College of Engineering, Beer Sheva 8428322, Israel.

Physics Department, Ben Gurion University of the Negev, Beer Sheva 8410501, Israel.

出版信息

Radiat Prot Dosimetry. 2023 Apr 19;199(6):498-508. doi: 10.1093/rpd/ncad032.

Abstract

A seeming contradiction in the prediction of the spatially correlated trapping center/luminescent center model applied to LiF:Mg,Ti has been the linear/supralinear behavior of the dose response of glow peak 5a. In the TC/LC model, the localised electron-hole recombination, giving rise to glow peak 5a, is expected to result in an extended region of linear dose response. Deconvolution of the glow curves based on first order kinetic peak shapes results, however, in a dose response of peak 5a, which closely resembles the linear/supralinear dose response of peak 5. It is demonstrated herein that when general-order kinetics peak shapes are used for peak 5a, the analysis can result in a linear dose response of glow peak 5a up to dose levels as high as 30 Gy, well beyond the 1-Gy onset of supralinearity of peak 5. The extended linearity suggests a resolution of the contradiction.

摘要

应用于 LiF:Mg,Ti 的空间相关俘获中心/发光中心模型的预测存在一个明显的矛盾,即 5a 发光峰的剂量响应呈线性/超线性。在 TC/LC 模型中,局部电子-空穴复合导致 5a 发光峰,预计会导致线性剂量响应的扩展区域。然而,基于一阶动力学峰形的发光曲线反卷积导致 5a 峰的剂量响应非常类似于 5 峰的线性/超线性剂量响应。本文证明,当使用一般阶动力学峰形来分析 5a 峰时,分析结果可以使 5a 发光峰的线性剂量响应高达 30Gy,远远超过 5 峰超线性的起始剂量 1Gy。这种扩展的线性性表明解决了这个矛盾。

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