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基于热和电可调过渡金属氧化物的等离子体光栅的红外辐射切换。

Infrared radiative switching with thermally and electrically tunable transition metal oxides-based plasmonic grating.

机构信息

Department of Mechanical Engineering, University of North Texas, Denton, 76207, USA.

School for Engineering of Matter, Transport & Energy, Arizona State University, Tempe, AZ, 85287, USA.

出版信息

Sci Rep. 2023 Mar 6;13(1):3702. doi: 10.1038/s41598-023-30959-4.

Abstract

Plasmonic and phase transition has been blended to gain the infrared radiative switching which is tunable with temperature or voltage supply. This is applied via vanadium dioxide, tungsten trioxide, and molybdenum trioxide as transition metal oxides (TMO). The metallic phase at high temperature or colored state contributes in magnetic polariton (MP) excitation, producing broad absorptance. The TMO-based sub-layer is integrated underneath the grating fully supporting MP resonance. In contrast, this underlayer leads to producing the narrowband absorptance originated from concept of zero contrast grating (ZCG). The zero gradient in refractive index at the output plane of the grating cause transmission of light in broad wavelength range. With introduction of reflective silver underlayer, those transmitted through the grating are reflected back. However, there exists the near-zero narrowband transmission peaks in ZCG. This undergoes transformation to narrowband absorptance. In addition, another absorptance peak can be induced due to phonon modes at insulating phase. The MP resonance at metallic phase is characterized with inductor-capacitor (LC) circuit and the narrowband absorptance peaks are characterized with phase shift from the Fabry-Perot round trip (FP-RT) eigenequation from high contrast grating (HCG). The work expands the usage of transition metal oxides in infrared region with larger contrast.

摘要

将等离子体和相变融合在一起,以获得可通过温度或电压供应调节的红外辐射开关。这是通过过渡金属氧化物(TMO),如二氧化钒、三氧化钨和三氧化钼来实现的。高温下的金属相或有色状态有助于磁极化激元(MP)激发,产生宽带吸收率。基于 TMO 的亚层完全集成在光栅下方,完全支持 MP 共振。相比之下,这种底层导致了源自零对比度光栅(ZCG)概念的窄带吸收率。光栅输出平面上折射率的零梯度导致在宽波长范围内传输光。通过引入反射性银底层,那些穿过光栅的光被反射回来。然而,在 ZCG 中存在近零的窄带透射峰。这会转变为窄带吸收率。此外,由于绝缘相的声子模式,还可以诱导另一个吸收率峰。金属相中的 MP 共振具有电感-电容(LC)电路的特性,而窄带吸收率峰则具有与高对比度光栅(HCG)的 Fabry-Perot 往返(FP-RT)本征方程的相位偏移的特性。这项工作扩展了过渡金属氧化物在红外区域的应用,具有更大的对比度。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f4a4/9988874/5c50b4895d66/41598_2023_30959_Fig1_HTML.jpg

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