School of Physics and Electronic Engineering, Jiangsu University, Zhenjiang, 212013, Jiangsu, China.
Jiangsu Engineering Research Center on Quantum Perception and Intelligent Detection of Agricultural Information, Zhenjiang, 212013, Jiangsu, China.
Nanoscale. 2023 May 18;15(19):8825-8831. doi: 10.1039/d3nr00651d.
Most special two-dimensional (2D) lattices, such as Kagome and Lieb lattices, can only generate a single flat band. Here, we propose a 2D lattice named a quadrangular-star lattice (QSL). It can produce coupling double flat bands, which indicates that there exists stronger electronic correlation than in the systems with only one flat band. Moreover, we suggest some 2D carbon allotropes ( CQSL-12 and CQSL-20), made of carbon rings and dimers, to realize QSL in real materials. By calculating the band structures of the carbon materials, we find that there are indeed two coupling flat bands around the Fermi level. Hole doping leads to strong magnetism of the carbon materials. When the two flat bands are half filled, , in the cases of one- and three-hole doping, the magnetic momentums mainly distribute on the atoms of the carbon rings and dimers, respectively. Even in the case of two-hole doping, the carbon structure also shows ferromagnetic characteristics, and the total magnetic moments are larger than the former two cases.
大多数特殊的二维(2D)晶格,如 Kagome 和 Lieb 晶格,只能产生单一的平带。在这里,我们提出了一种名为四角星晶格(QSL)的 2D 晶格。它可以产生耦合的双平带,这表明存在比只有一个平带的系统更强的电子关联。此外,我们建议了一些由碳环和二聚体组成的二维碳同素异形体(CQSL-12 和 CQSL-20),以在实际材料中实现 QSL。通过计算碳材料的能带结构,我们发现确实存在两个围绕费米能级的耦合平带。空穴掺杂导致碳材料具有强烈的磁性。当两个平带被半填充时,在单空穴和三空穴掺杂的情况下,磁动量主要分布在碳环和二聚体的原子上。即使在双空穴掺杂的情况下,碳结构也表现出铁磁特性,总磁矩大于前两种情况。