College of Environmental Science and Engineering, Ocean University of China, Qingdao 266003, China; Key Laboratory of Marine Environmental Science and Ecology, Ministry of Education, Ocean University of China, Qingdao, China.
College of Environmental Science and Engineering, Ocean University of China, Qingdao 266003, China; Key Laboratory of Marine Environmental Science and Ecology, Ministry of Education, Ocean University of China, Qingdao, China.
Sci Total Environ. 2023 Aug 10;885:163721. doi: 10.1016/j.scitotenv.2023.163721. Epub 2023 Apr 26.
Pharmaceutical and personal care products (PPCPs) were regarded as emerging environmental pollutants due to their ubiquitous appearance and high environmental risks. The wastewater treatment plants (WWTPs) became the hub of PPCPs receiving major sources of PPCPs used by humans. Increasing concern has been focused on promoting cost-effective ways to eliminate PPCPs within WWTPs for blocking their route into the environment through effluent discharging. Among all advanced technologies, constructed wetlands (CWs) with a combination of plants, substrates, and microbes attracted attention due to their cost-effectiveness and easier maintenance during long-term operation. This study offers baseline data for risk control and future treatment by discussing the extent and dispersion of PPCPs in surface waters over the past ten years and identifying the mechanisms of PPCPs removal in CWs based on the up-to-present research, with a special focus on the contribution of sediments, vegetation, and the interactions of microorganisms. The significant role of wetland plants in the removal of PPCPs was detailed discussed in identifying the contribution of direct uptake, adsorption, phytovolatilization, and biodegradation. Meanwhile, the correlation between the physical-chemical characteristics of PPCPs, the configuration operation of wetlands, as well as the environmental conditions with PPCP removal were also further estimated. Finally, the critical issues and knowledge gaps before the real application were addressed followed by promoted future works, which are expected to provide a comprehensive foundation for study on PPCPs elimination utilizing CWs and drive to achieve large-scale applications to treat PPCPs-contaminated surface waters.
药品和个人护理产品(PPCPs)因其广泛存在和高环境风险而被视为新兴的环境污染物。废水处理厂(WWTPs)成为接收人类使用的主要 PPCPs 源的中心。人们越来越关注在 WWTP 中通过消除废水排放来阻止 PPCPs 进入环境的有效且经济的方法,以促进消除 PPCPs。在所有先进技术中,植物、基质和微生物相结合的人工湿地(CWs)因其在长期运行过程中的成本效益和更易于维护而受到关注。本研究通过讨论过去十年地表水中国 PPCPs 的程度和分散情况,以及根据现有研究确定 CWs 中 PPCPs 去除的机制,为风险控制和未来处理提供了基线数据,特别关注沉积物、植被的贡献以及微生物的相互作用。湿地植物在去除 PPCPs 方面的重要作用在确定直接吸收、吸附、植物挥发和生物降解的贡献时进行了详细讨论。同时,还进一步估计了 PPCPs 的物理化学特性、湿地的配置操作以及与 PPCP 去除相关的环境条件之间的相关性。最后,针对实际应用之前的关键问题和知识空白进行了讨论,并提出了未来的工作,这有望为利用 CWs 去除 PPCPs 的研究提供全面的基础,并推动实现大规模应用来处理受 PPCPs 污染的地表水。