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SrCuBO 中近自由量子临界点

Proximate deconfined quantum critical point in SrCuBO.

机构信息

Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials and Micro-nano Devices, Renmin University of China, Beijing 100872, China.

Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.

出版信息

Science. 2023 Jun 16;380(6650):1179-1184. doi: 10.1126/science.adc9487. Epub 2023 May 25.

Abstract

The deconfined quantum critical point (DQCP) represents a paradigm shift in quantum matter studies, presenting a "beyond Landau" scenario for order-order transitions. Its experimental realization, however, has remained elusive. Using high-pressure B nuclear magnetic resonance measurements on the quantum magnet SrCu(BO), we here demonstrate a magnetic field-induced plaquette singlet to antiferromagnetic transition above 1.8 gigapascals at a notably low temperature, ≃ 0.07 kelvin. First-order signatures of the transition weaken with increasing pressure, and we observe quantum critical scaling at the highest pressure, 2.4 gigapascals. Supported by model calculations, we suggest that these observations can be explained by a proximate DQCP inducing critical quantum fluctuations and emergent O(3) symmetry of the order parameters. Our findings offer a concrete experimental platform for investigation of the DQCP.

摘要

无约束量子临界点(DQCP)代表了量子物质研究范式的转变,为有序-无序转变提供了一个“超越朗道”的情景。然而,其实验实现仍然难以捉摸。我们使用高压 B 核磁共振测量量子磁体 SrCu(BO),在这里证明了在显著低温 ≃ 0.07 开尔文下,磁场诱导的准单态到反铁磁转变在 1.8 吉帕斯卡以上。随着压力的增加,转变的一级特征减弱,我们在最高压力 2.4 吉帕斯卡下观察到量子临界标度。基于模型计算,我们提出这些观察结果可以用邻近的 DQCP 诱导临界量子涨落和序参量的涌现 O(3) 对称性来解释。我们的发现为研究 DQCP 提供了一个具体的实验平台。

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