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用于柔性透明导电电极的银纳米线沉积的多目标优化

Multiobjective Optimization of Silver-Nanowire Deposition for Flexible Transparent Conducting Electrodes.

作者信息

Lee Mark, Piper Robert T, Bhandari Bishal, Hsu Julia W P

机构信息

Department of Physics, University of Texas at Dallas, Richardson, Texas 75080, United States.

Department of Materials Science and Engineering, University of Texas at Dallas, Richardson, Texas 75080, United States.

出版信息

ACS Appl Nano Mater. 2023 Oct 2;6(19):17364-17368. doi: 10.1021/acsanm.3c03599. eCollection 2023 Oct 13.

DOI:10.1021/acsanm.3c03599
PMID:37854852
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10580235/
Abstract

Optimizing the spin coating of silver nanowires to form transparent conducting electrodes (TCE) is guided by machine learning (ML). A good TCE has two competing characteristics: high transmittance and high conductance. Optimization using a scalar figure of merit, as often done in the field, cannot satisfy the independent requirements for transmittance and conductance imposed by specific applications. By performing a Pareto front analysis based on ML models, we show that the desired outcomes of transmittance ≥ 75% and sheet resistance ≤ 15 Ω/sq are challenging but can be achieved using processing parameters identified by ML analysis.

摘要

利用机器学习指导银纳米线旋涂工艺以形成透明导电电极(TCE)。一个性能良好的TCE具有两个相互矛盾的特性:高透射率和高电导率。该领域通常采用标量品质因数进行优化,但无法满足特定应用对透射率和电导率的独立要求。通过基于机器学习模型进行帕累托前沿分析,我们表明,透射率≥75%且方阻≤15Ω/sq的理想结果具有挑战性,但可以使用机器学习分析确定的工艺参数来实现。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/197ba673b998/an3c03599_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/18a10312af20/an3c03599_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/58713757425b/an3c03599_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/197ba673b998/an3c03599_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/18a10312af20/an3c03599_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/58713757425b/an3c03599_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f7a6/10580235/197ba673b998/an3c03599_0003.jpg

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本文引用的文献

1
All-atmospheric fabrication of Ag-Cu core-shell nanowire transparent electrodes with Haacke figure of merit >600 × 10 Ω.具有哈克品质因数>600×10⁻³ Ω的Ag-Cu核壳纳米线透明电极的全大气制备。
Sci Rep. 2022 Dec 5;12(1):20962. doi: 10.1038/s41598-022-25080-x.
2
Advances in Flexible Metallic Transparent Electrodes.柔性金属透明电极的研究进展
Small. 2022 May;18(19):e2106006. doi: 10.1002/smll.202106006. Epub 2022 Feb 23.
3
High-performance silver nanowires transparent conductive electrodes fabricated using manufacturing-ready high-speed photonic sinterization solutions.
使用具备量产条件的高速光子烧结解决方案制造的高性能银纳米线透明导电电极。
Sci Rep. 2021 Dec 17;11(1):24156. doi: 10.1038/s41598-021-03528-w.
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Transparent conducting silver nanowire networks.透明导电银纳米线网络。
Nano Lett. 2012 Jun 13;12(6):3138-44. doi: 10.1021/nl301045a. Epub 2012 May 8.
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Silver Nanowire Networks as Flexible, Transparent, Conducting Films: Extremely High DC to Optical Conductivity Ratios.银纳米线网络作为灵活、透明、导电薄膜:极高的直流至光学电导率比。
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