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未来条件下臭氧与气温的关系:以中国四川盆地为例

Relationship between ozone and air temperature in future conditions: A case study in sichuan basin, China.

作者信息

Wang Ju, Li Juan, Li Xinlong, Wang Dali, Fang Chunsheng

机构信息

Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun 130021, China; Jilin Provincial Key Laboratory of Water Resources and Water Environment, Jilin University, Changchun 130021, China; College of New Energy and Environment, Jilin University, Changchun 130012, China.

Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun 130021, China; Jilin Provincial Key Laboratory of Water Resources and Water Environment, Jilin University, Changchun 130021, China; College of New Energy and Environment, Jilin University, Changchun 130012, China.

出版信息

Environ Pollut. 2024 Feb 15;343:123276. doi: 10.1016/j.envpol.2023.123276. Epub 2023 Dec 30.

Abstract

The Sichuan Basin (SCB) is located in southwestern China and has a unique topography where ozone (O) pollution is frequent during summer. Few studies have clarified the relationship between O and air temperature in SCB. Here, the SCB was divided into four major urban agglomerations. The weather research and forecasting model-community multiscale air quality model (WRF-CMAQ) was used to analyze the meteorology, spatial distribution characteristics of pollutants, and interactions among the urban agglomerations in the SCB. WRF-CMAQ was used to study the historical changes in the climate penalty factor (CPF) from 2015 to 2020 and the climate pathways under the SSP2-4.5 CPF in values in 2030 for the ambitious pollution NDC-goal scenario (NDC) and current-goals scenario (Current). The results show that the SCB is warmer in the summer months with prevailing northeasterly winds. Ozone accumulated in the western part of the SCB, and a high CPF of O concentration was most prominent in NW urban agglomeration, where the O concentration increased by 4.12-5.40 ppb for every 1 °C increase in air temperature. The observed CPF in the SCB in 2020 averaged 3.64 ppb/°C. The average CPF in the SCB in 2030 was 1.152 ppb/°C under the NDC scenario and 1.269 ppb/°C under the current scenario. This study is critical for understanding the relationship between O concentration and air temperature in China.

摘要

四川盆地位于中国西南部,地形独特,夏季臭氧(O₃)污染频发。很少有研究阐明四川盆地O₃与气温之间的关系。在此,将四川盆地划分为四个主要城市群。利用天气研究和预报模型-社区多尺度空气质量模型(WRF-CMAQ)分析四川盆地的气象学、污染物空间分布特征以及城市群之间的相互作用。利用WRF-CMAQ研究了2015年至2020年气候惩罚因子(CPF)的历史变化以及2030年在雄心勃勃的污染国家自主贡献目标情景(NDC)和当前目标情景(Current)下SSP2-4.5 CPF值的气候路径。结果表明,四川盆地夏季较为温暖,盛行东北风。臭氧在四川盆地西部积聚,O₃浓度的高CPF在西北城市群最为突出,那里气温每升高1℃,O₃浓度增加4.12 - 5.40 ppb。2020年四川盆地观测到的CPF平均为3.64 ppb/℃。在NDC情景下,2030年四川盆地的平均CPF为1.152 ppb/℃,在当前情景下为1.269 ppb/℃。本研究对于理解中国O₃浓度与气温之间的关系至关重要。

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