Wang Ju, Li Juan, Li Xinlong, Wang Dali, Fang Chunsheng
Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun 130021, China; Jilin Provincial Key Laboratory of Water Resources and Water Environment, Jilin University, Changchun 130021, China; College of New Energy and Environment, Jilin University, Changchun 130012, China.
Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun 130021, China; Jilin Provincial Key Laboratory of Water Resources and Water Environment, Jilin University, Changchun 130021, China; College of New Energy and Environment, Jilin University, Changchun 130012, China.
Environ Pollut. 2024 Feb 15;343:123276. doi: 10.1016/j.envpol.2023.123276. Epub 2023 Dec 30.
The Sichuan Basin (SCB) is located in southwestern China and has a unique topography where ozone (O) pollution is frequent during summer. Few studies have clarified the relationship between O and air temperature in SCB. Here, the SCB was divided into four major urban agglomerations. The weather research and forecasting model-community multiscale air quality model (WRF-CMAQ) was used to analyze the meteorology, spatial distribution characteristics of pollutants, and interactions among the urban agglomerations in the SCB. WRF-CMAQ was used to study the historical changes in the climate penalty factor (CPF) from 2015 to 2020 and the climate pathways under the SSP2-4.5 CPF in values in 2030 for the ambitious pollution NDC-goal scenario (NDC) and current-goals scenario (Current). The results show that the SCB is warmer in the summer months with prevailing northeasterly winds. Ozone accumulated in the western part of the SCB, and a high CPF of O concentration was most prominent in NW urban agglomeration, where the O concentration increased by 4.12-5.40 ppb for every 1 °C increase in air temperature. The observed CPF in the SCB in 2020 averaged 3.64 ppb/°C. The average CPF in the SCB in 2030 was 1.152 ppb/°C under the NDC scenario and 1.269 ppb/°C under the current scenario. This study is critical for understanding the relationship between O concentration and air temperature in China.
四川盆地位于中国西南部,地形独特,夏季臭氧(O₃)污染频发。很少有研究阐明四川盆地O₃与气温之间的关系。在此,将四川盆地划分为四个主要城市群。利用天气研究和预报模型-社区多尺度空气质量模型(WRF-CMAQ)分析四川盆地的气象学、污染物空间分布特征以及城市群之间的相互作用。利用WRF-CMAQ研究了2015年至2020年气候惩罚因子(CPF)的历史变化以及2030年在雄心勃勃的污染国家自主贡献目标情景(NDC)和当前目标情景(Current)下SSP2-4.5 CPF值的气候路径。结果表明,四川盆地夏季较为温暖,盛行东北风。臭氧在四川盆地西部积聚,O₃浓度的高CPF在西北城市群最为突出,那里气温每升高1℃,O₃浓度增加4.12 - 5.40 ppb。2020年四川盆地观测到的CPF平均为3.64 ppb/℃。在NDC情景下,2030年四川盆地的平均CPF为1.152 ppb/℃,在当前情景下为1.269 ppb/℃。本研究对于理解中国O₃浓度与气温之间的关系至关重要。