Qian Yongteng, Zhang Fangfang, Luo Xiaohui, Zhong Yijun, Kang Dae Joon, Hu Yong
Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Department of Chemistry, Zhejiang Normal University, Jinhua, 321004, P. R. China.
College of Pharmacy, Jinhua Polytechnic, Jinhua, Zhejiang, 321007, P. R. China.
Small. 2024 Jun;20(26):e2310526. doi: 10.1002/smll.202310526. Epub 2024 Jan 14.
Featured with the attractive properties such as large surface area, unique atomic layer thickness, excellent electronic conductivity, and superior catalytic activity, layered metal chalcogenides (LMCs) have received considerable research attention in electrocatalytic applications. In this review, the approaches developed to synthesize LMCs-based electrocatalysts are summarized. Recent progress in LMCs-based composites for electrochemical energy conversion applications including oxygen reduction reaction, carbon dioxide reduction reaction, oxygen evolution reaction, hydrogen evolution reaction, overall water splitting, and nitrogen reduction reaction is reviewed, and the potential opportunities and practical obstacles for the development of LMCs-based composites as high-performing active substances for electrocatalytic applications are also discussed. This review may provide an inspiring guidance for developing high-performance LMCs for electrochemical energy conversion applications.
层状金属硫族化合物(LMCs)具有大表面积、独特的原子层厚度、优异的电子导电性和卓越的催化活性等吸引人的特性,在电催化应用中受到了广泛的研究关注。在这篇综述中,总结了用于合成基于LMCs的电催化剂的方法。综述了基于LMCs的复合材料在包括氧还原反应、二氧化碳还原反应、析氧反应、析氢反应、全水分解和氮还原反应在内的电化学能量转换应用中的最新进展,并讨论了将基于LMCs的复合材料开发为电催化应用的高性能活性物质的潜在机遇和实际障碍。这篇综述可能为开发用于电化学能量转换应用的高性能LMCs提供启发性的指导。