Pacific Northwest National Laboratory, Richland, WA 99352, USA; WSU-PNNL Bioproducts Institute, WA 99352, USA.
Systems Assessment Center, Argonne National Laboratory, Lemont, IL 60439, USA.
Bioresour Technol. 2024 Apr;397:130504. doi: 10.1016/j.biortech.2024.130504. Epub 2024 Feb 27.
While wet waste hydrothermal liquefaction technology has a high biofuel yield, a significant amount of the carbon and nitrogen in the feedstock reports to the aqueous-phase product. Pretreatment of this stream before sending to a conventional wastewater plant is essential or at the very least, advisable. In this work, techno-economic and life-cycle assessments were conducted for the state-of-technology baseline and four aqueous-phase product treatment and monetization options based on experimental data. These options can cut minimum fuel selling prices by up to 13 % and life-cycle greenhouse gas emissions by up to 39 % compared to the baseline. These findings highlight the substantial influence of aqueous produce treatment strategies on the entire wet waste hydrothermal liquefaction process, demonstrating the potential for optimizing economic viability and environmental impact through further research and development of milder treatment methods and diversified by-product valorization pathways.
尽管湿废物水热液化技术具有较高的生物燃料产率,但原料中相当一部分的碳和氮会转移到水相产物中。在将该物流输送到传统废水厂之前,对其进行预处理是必不可少的,或者至少是明智的。在这项工作中,根据实验数据,对技术现状基准以及基于四种水相产物处理和货币化选择进行了技术经济和生命周期评估。与基准相比,这些选择可以将最低燃料销售价格降低多达 13%,并将生命周期温室气体排放减少多达 39%。这些发现强调了水相产物处理策略对整个湿废物水热液化过程的重大影响,表明通过进一步研究和开发更温和的处理方法以及通过多样化的副产品增值途径,可以优化经济可行性和环境影响。