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高温下金属 Kagome 铁磁体 FeSn 的各向同性本质

Isotropic Nature of the Metallic Kagome Ferromagnet FeSn at High Temperatures.

作者信息

Dally Rebecca L, Phelan Daniel, Bishop Nicholas, Ghimire Nirmal J, Lynn Jeffrey W

机构信息

NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, MD 20899-6102.

Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439.

出版信息

Crystals (Basel). 2021;11(3). doi: 10.3390/cryst11030307.

Abstract

Anisotropy and competing exchange interactions have emerged as two central ingredients needed for centrosymmetric materials to exhibit topological spin textures. FeSn is thought to have these ingredients as well, as it has recently been discovered to host room temperature skyrmionic bubbles with an accompanying topological Hall effect. We present small-angle inelastic neutron scattering measurements that unambiguously show that FeSn is an isotropic ferromagnet below to at least 480 K - the lower temperature threshold of our experimental configuration. FeSn is known to have competing magnetic exchange interactions, correlated electron behavior, weak magnetocrystalline anisotropy, and lattice anisotropy; all of these features are thought to play a role in stabilizing skyrmions in centrosymmetric systems. Our results reveal that at elevated temperatures, there is an absence of magnetocrystalline anisotropy and that the system behaves as a typical exchange ferromagnet with a spin stiffness .

摘要

各向异性和竞争交换相互作用已成为中心对称材料展现拓扑自旋纹理所需的两个核心要素。人们认为FeSn也具备这些要素,因为最近发现它在室温下能形成伴随拓扑霍尔效应的斯格明子气泡。我们进行了小角非弹性中子散射测量,结果明确表明,在至少480K以下(这是我们实验装置的较低温度阈值),FeSn是一种各向同性铁磁体。已知FeSn具有竞争磁交换相互作用、关联电子行为、弱磁晶各向异性和晶格各向异性;所有这些特征都被认为在中心对称系统中斯格明子的稳定过程中发挥作用。我们的结果表明,在高温下,磁晶各向异性不存在,且该系统表现为具有自旋刚度的典型交换铁磁体。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2db5/10938373/ec37bba977c6/nihms-1918195-f0001.jpg

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