Xu Sen, Li Si-Liang, Bufe Aaron, Klaus Marcus, Zhong Jun, Wen Hang, Chen Shuai, Li Li
Institute of Surface-Earth System Sciences, School of Earth System Science, Tianjin University, Tianjin 300072, China.
Department of Earth and Environmental Sciences, Ludwig-Maximilians-Universität München, Munich 80333, Germany.
Environ Sci Technol. 2024 Apr 23;58(16):7032-7044. doi: 10.1021/acs.est.3c06777. Epub 2024 Apr 11.
High-elevation mountains have experienced disproportionately rapid warming, yet the effect of warming on the lateral export of terrestrial carbon to rivers remains poorly explored and understood in these regions. Here, we present a long-term data set of dissolved inorganic carbon (DIC) and a more detailed, short-term data set of DIC, δC, and organic carbon from two major rivers of the Qinghai-Tibetan Plateau, the Jinsha River (JSR) and the Yalong River (YLR). In the higher-elevation JSR with ∼51% continuous permafrost coverage, warming (>3 °C) and increasing precipitation coincided with substantially increased DIC concentrations by 35% and fluxes by 110%. In the lower-elevation YLR with ∼14% continuous permafrost, such increases did not occur despite a comparable extent of warming. Riverine concentrations of dissolved and particulate organic carbon increased with discharge (mobilization) in both rivers. In the JSR, DIC concentrations transitioned from dilution (decreasing concentration with discharge) in earlier, colder years to chemostasis (relatively constant concentration) in later, warmer years. This changing pattern, together with lighter δC under high discharge, suggests that permafrost thawing boosts DIC production and export via enhancing soil respiration and weathering. These findings reveal the predominant role of warming in altering carbon lateral export by escalating concentrations and fluxes and modifying export patterns.
高海拔山区经历了异常迅速的变暖,但在这些地区,变暖对陆地碳向河流的侧向输出的影响仍未得到充分研究和理解。在此,我们展示了青藏高原两条主要河流——金沙江(JSR)和雅砻江(YLR)的溶解无机碳(DIC)长期数据集,以及更详细的DIC、δC和有机碳短期数据集。在多年冻土覆盖率约为51%的高海拔金沙江,变暖(>3°C)和降水增加的同时,DIC浓度大幅增加了35%,通量增加了110%。在多年冻土覆盖率约为14%的低海拔雅砻江,尽管变暖程度相当,但并未出现这种增加。两条河流中溶解有机碳和颗粒有机碳的河流浓度均随流量(搬运)增加。在金沙江,DIC浓度从早期较冷年份的稀释(浓度随流量降低)转变为后期较暖年份的化学稳定(浓度相对恒定)。这种变化模式,以及高流量下较轻的δC,表明多年冻土融化通过增强土壤呼吸和风化促进了DIC的产生和输出。这些发现揭示了变暖在通过提高浓度和通量以及改变输出模式来改变碳侧向输出方面的主导作用。