He De-Chun, Zheng Mi-Mi, Huang Wei, Liu Wang-Rong, Hu Jia-Wu, Liu Jiang-Yan, Pan Jie
College of Environmental and Chemical Engineering, Chongqing Three Gorges University, Chongqing 404000, China.
South China Institute of Environmental Sciences, Ministry of Ecology and Environment, Guangzhou 510530, China.
Huan Jing Ke Xue. 2024 Jun 8;45(6):3247-3259. doi: 10.13227/j.hjkx.202305189.
Pharmaceuticals and personal care products (PPCPs) have received extensive attention as a new type of pollutant inin the 21st century, and the ecological and health risks caused by PPCPs have gradually been recognized by government regulatory agencies. Daily use of PPCPs has led to their frequent detection and high concentrations in the influent, effluent, and sludge of wastewater treatment plants, but traditional wastewater treatment processes can't remove them effectively. Most research about enhancing the removal of PPCPs through microbial degradation, photodegradation, and ozonation is still in the laboratory research stage, and the removal effects are not satisfactory when applied to actual sewage treatment. Therefore, the effective removal of PPCPs from domestic wastewater is a critical technical problem that urgently needs to be studied and solved in the coming years. At present, many scholars do not have a comprehensive understanding about the degradation and transformation behaviors of microbes, ultraviolet, and ozone for typical PPCPs in the wastewater treatment process, so it is necessary to conduct a systematic analysis and discussion. In this study, 16 typical PPCPs frequently detected in sewage treatment plants were selected as research objects through a literature review. The occurrence, removal characteristics, and sludge adsorption properties of typical PPCPs in wastewater treatment plants were analyzed and summarized. The degradation and transformation behavior of typical PPCPs under microbial, ultraviolet, and ozone treatments in the wastewater treatment process were also discussed. Finally, based on current research gaps, some research directions for the removal and transformation of PPCPs in wastewater were proposed:① investigation into the removal characteristics of PPCPs by actual biochemical treatment; ② study on the mechanism of microbial degradation and transformation of typical PPCPs during biochemical treatment; ③ study on the degradation and transformation mechanism of typical PPCPs by UV/ozone in an actual sewage system; and ④ research on the application technology of removing PPCPs from sewage via microbial degradation, photodegradation, ozone oxidation, etc. The relevant results of this study can provide a reference for the pollution control of typical PPCPs in the sewage treatment process.
药品和个人护理产品(PPCPs)作为21世纪的一种新型污染物受到了广泛关注,PPCPs所造成的生态和健康风险已逐渐得到政府监管机构的认可。PPCPs的日常使用导致它们在污水处理厂的进水、出水和污泥中被频繁检测到且浓度较高,但传统的污水处理工艺无法有效去除它们。大多数关于通过微生物降解、光降解和臭氧化来提高PPCPs去除率的研究仍处于实验室研究阶段,应用于实际污水处理时去除效果并不理想。因此,从生活污水中有效去除PPCPs是未来几年迫切需要研究和解决的关键技术问题。目前,许多学者对污水处理过程中微生物、紫外线和臭氧对典型PPCPs的降解和转化行为缺乏全面了解,因此有必要进行系统的分析和讨论。本研究通过文献综述,选取了污水处理厂中经常检测到的16种典型PPCPs作为研究对象。分析和总结了典型PPCPs在污水处理厂中的存在情况、去除特性和污泥吸附特性。还讨论了典型PPCPs在污水处理过程中微生物、紫外线和臭氧处理下的降解和转化行为。最后,基于当前的研究差距,提出了一些关于废水中PPCPs去除和转化的研究方向:①实际生化处理对PPCPs的去除特性研究;②生化处理过程中典型PPCPs的微生物降解和转化机制研究;③实际污水系统中紫外线/臭氧对典型PPCPs的降解和转化机制研究;④通过微生物降解、光降解、臭氧氧化等方法从污水中去除PPCPs的应用技术研究。本研究的相关结果可为污水处理过程中典型PPCPs的污染控制提供参考。