Oak Ridge Institute for Science and Education, Oak Ridge, TN, 37830, USA.
Ohio Agricultural Research and Development Center, School of Environment and Natural Resources, The Ohio State University, Wooster, OH, 44691, USA.
Sci Data. 2024 Jun 29;11(1):712. doi: 10.1038/s41597-024-03552-1.
Riverine nitrogen is a pivotal determinant influencing water quality in inland and coastal waters. Despite the recognized utility, no spatially-explicit data on riverine nitrogen yield is available for large parts of the world, thus hindering our ability to identify the contributors to riverine nitrogen and understand aquatic nitrogen cycling. To fill the data gap for the United States, here we (1) compiled 294,996 total nitrogen (TN), 225,827 nitrate (NO), 204,015 ammonium (NH), and 158,837 total organic nitrogen (TON) concentrations, with concurrent streamflow data, across the Conterminous United States (CONUS), (2) estimated riverine nitrogen loads for over 1,800 hydrological stations, (3) derived the spatial distribution of annual riverine nitrogen yield by leveraging river and catchment connectivity information contained in the National Hydrography Dataset plus (NHDPlus), and (4) characterized nonpoint-source TN loads by excluding point-source loads. This new spatial dataset quantifies spatial sources of nitrogen yield from point and non-point sources (e.g., up to 36% from point sources across the U.S.) and serves as ground-truthing to validate water quality models.
河川氮是影响内陆和沿海水质的关键决定因素。尽管已经认识到其重要性,但世界上很大一部分地区仍缺乏关于河川氮输出的空间明确数据,从而阻碍了我们识别河川氮的贡献者和了解水生氮循环的能力。为了填补美国的数据空白,我们(1)汇编了美国大陆(CONUS)范围内的 294996 个总氮(TN)、225827 个硝酸盐(NO3)、204015 个铵(NH4)和 158837 个总有机氮(TON)浓度,以及同期的流量数据,(2)估计了超过 1800 个水文站的河川氮负荷,(3)通过利用包含在国家水文数据集 plus(NHDPlus)中的河流和流域连通性信息,推导出了年度河川氮输出的空间分布,(4)通过排除点源负荷,描述了非点源 TN 负荷。这个新的空间数据集量化了氮输出的空间来源,包括点源和非点源(例如,美国各地的点源占比高达 36%),并为水质模型提供了验证。