Chen Jiachuan, Wang Xiaofa, Wang Baobin, Wu Ting, Zhang Lei, Zhang Kai, Fang Guigan, Wang Yueying, Zhao Yu, Yang Guihua
State Key Laboratory of Biobased Material and Green Papermaking, Qilu University of Technology, Shandong Academy of Sciences, Jinan, 250353, China.
Institute of Chemical Industry of Forest Products, Chinese Academy of Forestry, Nanjing, Jiangsu Province, 210042, China.
Small. 2024 Nov;20(47):e2403221. doi: 10.1002/smll.202403221. Epub 2024 Jul 16.
Solar interfacial evaporation strategy (SIES) has shown great potential to deal with water scarcity and energy crisis. Biobased hydrogel derived interfacial evaporator can realize efficient evaporation due to the unique structure- properties relationship. As such, increasing studies have focused on water treatment or even potential accompanying advanced energy storage applications with respect of efficiency and mechanism of bio-based hydrogel derived interfacial evaporation from microscale to molecular scale. In this review, the interrelationship between efficient interfacial evaporator and bio-based hydrogel is first presented. Then, special attention is paid on the inherent molecular characteristics of the biopolymer related to the up-to-date studies of promising biopolymers derived interfacial evaporator with the objective to showcase the unique superiority of biopolymer. In addition, the applications of the bio-based hydrogels are highlighted concerning the aspects including water desalination, water decontamination atmospheric water harvesting, energy storage and conversion. Finally, the challenges and future perspectives are given to unveil the bottleneck of the biobased hydrogel derived SIES in sustainable water and other energy storage applications.
太阳能界面蒸发策略(SIES)在应对水资源短缺和能源危机方面已展现出巨大潜力。基于生物基水凝胶的界面蒸发器由于独特的结构-性能关系能够实现高效蒸发。因此,越来越多的研究聚焦于从微观尺度到分子尺度的基于生物基水凝胶的界面蒸发效率及机理的水处理甚至潜在的伴随先进储能应用。在本综述中,首先阐述了高效界面蒸发器与生物基水凝胶之间的相互关系。然后,特别关注与有前景的基于生物聚合物的界面蒸发器最新研究相关的生物聚合物的固有分子特性,目的是展示生物聚合物的独特优势。此外,还突出了生物基水凝胶在海水淡化、水净化、大气取水、储能和能量转换等方面的应用。最后,给出了挑战和未来展望,以揭示基于生物基水凝胶的SIES在可持续水及其他储能应用中的瓶颈。