Sun Mingrui, Glenn Chase K, El Hajj Omar, Kumar Kruthika V, Anosike Anita, Penland Robert, Callaham Mac A, Loudermilk E Louise, O'Brien Joseph J, Saleh Rawad, Smith Geoffrey D
Department of Chemistry, University of Georgia, Athens, Georgia 30602, United States.
School of Environmental, Civil, Agricultural and Mechanical Engineering, University of Georgia, Athens, Georgia 30602, United States.
ACS EST Air. 2024 Jul 10;1(9):989-999. doi: 10.1021/acsestair.4c00016. eCollection 2024 Sep 13.
This work, as part of the Georgia Wildland fire Simulation Experiment (G-WISE) campaign, explores the aqueous photolysis of water-soluble brown carbon (W-BrC) in biomass burning aerosols from the combustion of fuel beds collected from three distinct ecoregions in Georgia: Piedmont, Coastal Plain, and Blue Ridge. Burns were conducted under conditions representative of wildfires, which are common unplanned occurrences in Southeastern forests (low fuel moisture content), and prescribed fires, which are commonly used in forest management (higher fuel moisture content). Upon exposure to radiation from UV lamps equivalent to approximately 5 h in the atmosphere, the absorption spectra of all six samples exhibited up to 40% photobleaching in the UV range (280-400 nm) and as much as 30% photo-enhancement in the visible range (400-500 nm). Together, these two effects reduced the absorption Ångström exponent (AAE), a measure of the wavelength dependence of the spectrum, from 6.0-7.9 before photolysis to 5.0-5.7 after. Electrospray ionization ultrahigh-resolution mass spectrometry analysis shows the potential formation of oligomeric chromophores due to aqueous photolysis. This work provides insight into the impacts that aqueous photolysis has on W-BrC in biomass burning aerosols and its dependence on fuel bed composition and moisture content.
这项工作作为佐治亚州野火模拟实验(G-WISE)活动的一部分,探究了来自佐治亚州三个不同生态区域(皮埃蒙特、沿海平原和蓝岭)收集的燃料床燃烧产生的生物质燃烧气溶胶中水溶性棕碳(W-BrC)的水相光解。燃烧实验是在代表野火(东南部森林中常见的意外火灾,燃料含水量低)和规定火烧(森林管理中常用,燃料含水量高)的条件下进行的。在暴露于相当于大气中约5小时的紫外灯辐射后,所有六个样品的吸收光谱在紫外范围(280 - 400 nm)显示出高达40%的光漂白,在可见光范围(400 - 500 nm)显示出高达30%的光增强。这两种效应共同作用,使吸收埃指数(AAE,光谱波长依赖性的一种度量)从光解前的6.0 - 7.9降低到光解后的5.0 - 5.7。电喷雾电离超高分辨率质谱分析表明,水相光解可能会形成低聚发色团。这项工作深入了解了水相光解对生物质燃烧气溶胶中W-BrC的影响及其对燃料床组成和含水量的依赖性。