Kim Howon, Morr Dirk K, Wiesendanger Roland
Department of Physics, University of Hamburg, D-20355 Hamburg, Germany.
Department of Physics, University of Illinois at Chicago, Chicago, Illinois 60607, United States.
Nano Lett. 2024 Nov 6;24(44):14139-14145. doi: 10.1021/acs.nanolett.4c04796. Epub 2024 Oct 25.
Realizing hybrids of low-dimensional Kondo lattices and superconducting substrates leads to fascinating platforms for studying the exciting physics of strongly correlated electron systems with induced superconducting pairing. Here, we report a scanning tunneling microscopy and spectroscopy study of a new type of two-dimensional (2D) La-Ce alloy grown epitaxially on a superconducting Re(0001) substrate. We observe the characteristic spectroscopic signature of a hybridization gap evidencing the coherent spin screening in the 2D Kondo lattice realized by the ultrathin La-Ce alloy film on normal conducting Re(0001). Upon lowering the temperature below the critical temperature of rhenium, a superconducting gap is induced exhibiting an energy asymmetry of the coherence peaks that arises from the interaction of residual unscreened magnetic moments with the superconducting substrate. A positive correlation between the Kondo hybridization gap and the asymmetry of the coherence peaks is found.
实现低维近藤晶格与超导衬底的杂化,为研究具有诱导超导配对的强关联电子系统的激动人心的物理特性提供了引人入胜的平台。在此,我们报告了一项关于在超导Re(0001)衬底上外延生长的新型二维(2D) La-Ce合金的扫描隧道显微镜和光谱研究。我们观察到杂化能隙的特征光谱特征,这证明了在正常导电的Re(0001)上由超薄La-Ce合金膜实现的二维近藤晶格中的相干自旋筛选。当温度降低到铼的临界温度以下时,会诱导出一个超导能隙,该能隙表现出相干峰的能量不对称性,这是由残余未屏蔽磁矩与超导衬底的相互作用引起的。我们发现近藤杂化能隙与相干峰的不对称性之间存在正相关。