College of Nuclear Science and Technology, Harbin Engineering University, Harbin, 150001, China; Thamar University, Faculty of Science, Department of Physics, Yemen; National Atomic Energy Commission-Yemen (NATEC), Sana'a, Yemen.
National Atomic Energy Commission-Yemen (NATEC), Sana'a, Yemen; Faculty of Education, University of Aden, Yemen.
Appl Radiat Isot. 2025 Jan;215:111566. doi: 10.1016/j.apradiso.2024.111566. Epub 2024 Oct 28.
This study was conducted in Lahij city, Yemen, to evaluate the concentrations and potential health risks of natural radioactive nuclides and heavy metals in soil and drinking water. A total of 21 soil samples and 17 water samples were collected from various locations. A high-purity germanium gamma detector HPGe was used to measure the concentrations of K, Th, and Ra in all samples, along with the concentrations of heavy metals. In soil samples, the average concentrations of K, Th, and Ra were 731.5, 30.7, and 28.16 Bq kg, respectively. While some samples showed higher than permissible levels for Ra and Th, the overall average remained within acceptable limits. However, K levels were almost twice the recommended global limits. In water samples, the average concentrations of these nuclides were 5.38, 0.73, and 0.66 Bq L, all within the global safety limits. Radiological risk assessments for soil indicated an average radium equivalent activity (Ra) of 124.4 Bq kg, absorbed dose rate in air of 59.9 nGy h, annual effective dose rate of 0.07 mSv y, outdoor excess lifetime cancer risk (ELCR) of 0.26 × 10, and annual gonad equivalent dose (AGED) of 336.6 mSv y. Risk indices, including the activity concentration index (I), external hazard index (H), and internal hazard index (H), averaged 0.48, 0.34, and 0.41, respectively, all below global limits except for AGED, which slightly exceeded the recommended level. For drinking water, the total ingestion dose was calculated for different age groups. The average doses for infants, children, and adults were 0.15, 0.27, and 0.19 mSv y, respectively. The doses for children and adults exceeded the permissible limits, while those for infants were within safe levels. Heavy metal concentrations were measured in all samples, and the Hazard Quotient (HQ) was calculated. In soil samples, HQ values for all metals >1, indicating potential health risks. In water samples, HQ values were also >1 for all metals except vanadium (V) and iron (Fe). To reduce the dangers associated with radioactive nuclides and heavy metals, regular monitoring and cleanup are crucial, and further research is needed to understand contamination sources and long-term health impacts.
这项研究在也门拉哈吉市进行,旨在评估土壤和饮用水中天然放射性核素和重金属的浓度及其潜在健康风险。共采集了 21 个土壤样本和 17 个水样,来自不同地点。使用高纯锗伽马探测器 HPGe 测量了所有样本中 K、Th 和 Ra 的浓度,以及重金属的浓度。在土壤样本中,K、Th 和 Ra 的平均浓度分别为 731.5、30.7 和 28.16 Bq kg。虽然一些样本的 Ra 和 Th 浓度超过了允许水平,但总体平均值仍在可接受范围内。然而,K 水平几乎是全球推荐限值的两倍。在水样中,这些核素的平均浓度分别为 5.38、0.73 和 0.66 Bq L,均在全球安全限值范围内。土壤的辐射风险评估表明,平均镭当量活度(Ra)为 124.4 Bq kg,空气中的吸收剂量率为 59.9 nGy h,年有效剂量率为 0.07 mSv y,室外超额终生癌症风险(ELCR)为 0.26×10,年性腺当量剂量(AGED)为 336.6 mSv y。风险指数包括活度浓度指数(I)、外照射指数(H)和内照射指数(H),平均值分别为 0.48、0.34 和 0.41,除 AGED 略微超过推荐水平外,均低于全球限值。对于饮用水,计算了不同年龄组的总摄入剂量。婴儿、儿童和成人的平均剂量分别为 0.15、0.27 和 0.19 mSv y。儿童和成人的剂量超过了允许水平,而婴儿的剂量处于安全水平。所有样本都测量了重金属浓度,并计算了危害系数(HQ)。在土壤样本中,所有金属的 HQ 值均>1,表明存在潜在的健康风险。在水样中,除钒(V)和铁(Fe)外,所有金属的 HQ 值也>1。为了降低放射性核素和重金属带来的危险,定期监测和清理至关重要,还需要进一步研究以了解污染来源和长期健康影响。