Gangemi Roberto, Bignotti Mattia, Denardo Andrea, Pearce Claudia N, Ronzoni Riccardo, Lomas David A, Irving James A, Fra Annamaria, Gangemi Fabrizio
Physics, Department of Molecular and Translational Medicine, University of Brescia, Italy.
Experimental Oncology and Immunology, Department of Molecular and Translational Medicine, University of Brescia, Italy.
FEBS J. 2025 Apr;292(8):1887-1903. doi: 10.1111/febs.17387. Epub 2025 Jan 8.
Neutrophil elastase (NE) is released by activated neutrophils during an inflammatory response and exerts proteolytic activity on elastin and other extracellular matrix components. This protease is rapidly inhibited by the plasma serine protease inhibitor alpha-1-antitrypsin (AAT), and the importance of this protective activity on lung tissue is highlighted by the development of early onset emphysema in individuals with AAT deficiency. As a serpin, AAT presents a surface-exposed reactive centre loop (RCL) whose sequence mirrors the target protease specificity. Following binding of NE in a 'Michaelis' encounter complex, cleavage of the RCL results in an irreversible complex between the two molecules. Here, the structure of the AAT-NE encounter complex was studied by molecular dynamics, mutagenesis and enzyme kinetics. Exploration of the geometry of interaction between the two molecules revealed the possibility that the interaction interface extends beyond the RCL; a persistent feature of the simulations was the interaction between a region located upstream of β-strand 4C of AAT, comprising three acidic residues (Asp202, Glu199 and Glu204), and Arg147 of NE. Mutation of the acidic residues to either alanine or serine, or a D202R substitution, resulted in a reduced rate of association between recombinant AAT and NE. Addition of salt to the buffer had little effect for these mutants but substantially reduced the rate of interaction of the wild-type protein. These data are consistent with a role for this acidic region on AAT as an exosite that contributes to an optimal interaction with its physiological protease target.
中性粒细胞弹性蛋白酶(NE)在炎症反应期间由活化的中性粒细胞释放,并对弹性蛋白和其他细胞外基质成分发挥蛋白水解活性。这种蛋白酶会被血浆丝氨酸蛋白酶抑制剂α-1-抗胰蛋白酶(AAT)迅速抑制,AAT缺乏个体中早发性肺气肿的发生突出了这种对肺组织的保护活性的重要性。作为一种丝氨酸蛋白酶抑制剂,AAT呈现出一个表面暴露的反应中心环(RCL),其序列反映了靶蛋白酶的特异性。在“米氏”相遇复合物中NE结合后,RCL的切割导致两个分子之间形成不可逆的复合物。在此,通过分子动力学、诱变和酶动力学研究了AAT-NE相遇复合物的结构。对两个分子之间相互作用几何结构的探索揭示了相互作用界面可能延伸超出RCL的可能性;模拟的一个持续特征是AAT的β链4C上游区域(包含三个酸性残基(Asp202、Glu199和Glu204))与NE的Arg147之间的相互作用。将酸性残基突变为丙氨酸或丝氨酸,或进行D202R替换,导致重组AAT与NE之间的结合速率降低。向缓冲液中添加盐对这些突变体影响不大,但显著降低了野生型蛋白的相互作用速率。这些数据与AAT上的这个酸性区域作为一个外部位点的作用一致,该位点有助于与其生理蛋白酶靶标进行最佳相互作用。