Lai Joey, Bahri Carlota, Truong Mai P, Downey Kathleen T, Sammis Glenn M
Department of Chemistry, The University of British Columbia, 2036 Main Mall, Vancouver, BC, V6T 1Z1, Canada.
Commun Chem. 2025 Feb 22;8(1):53. doi: 10.1038/s42004-025-01456-8.
Peptide couplings have been a subject of investigation for over a century, with modern research seeking to discover new methodologies that minimize purification steps, minimize reagent expense, and/or decrease reaction times. Of the numerous coupling reagents available, sulfur(IV) fluorides have potential as they can effectively transform carboxylic acids to reactive intermediates, and the sulfite by-products can be removed through aqueous washes. Here we demonstrate the formation and capture of key acyl fluorosulfite intermediates for peptide couplings in 15 min total, without epimerization or column chromatography for purification. Dipeptides were obtained in 40-94% yields. This approach was expanded to longer chains through iterative couplings, with oligopeptides obtained in 24-57% yields, each within 2 days. Mechanistic studies indicate the reaction does not proceed through acyl fluoride intermediates, and instead involves nucleophilic catalysis. The mild conditions are tolerant of a wide range of protecting groups of canonical and non-canonical amino acids.
肽偶联反应已被研究了一个多世纪,现代研究致力于发现新的方法,以尽量减少纯化步骤、降低试剂成本和/或缩短反应时间。在众多可用的偶联试剂中,四价硫氟化物具有潜力,因为它们可以有效地将羧酸转化为活性中间体,并且亚硫酸盐副产物可以通过水洗去除。在此,我们展示了在总共15分钟内形成并捕获用于肽偶联的关键酰基氟亚硫酸盐中间体,无需差向异构化或柱色谱纯化。二肽的产率为40 - 94%。通过迭代偶联将该方法扩展到更长的链,寡肽的产率为24 - 57%,且均在2天内完成。机理研究表明该反应不是通过酰氟中间体进行的,而是涉及亲核催化。温和的条件对多种标准和非标准氨基酸的保护基团具有耐受性。