Elsafi Mohamed, Hanfi Mohamed Y, Al-Balawi Shoaa M, Sayyed M I
Physics Department, Faculty of Science, Alexandria University, Alexandria, 21511, Egypt.
Ural Federal University, Ekaterinburg, 620002, Russia.
Sci Rep. 2025 Jun 27;15(1):20321. doi: 10.1038/s41598-025-05275-8.
In this study, the integration of PbO into a borosilicate glass system was investigated for enhanced radiation shielding performance. Several glasses with varying PbO concentrations (31, 33, 35 and 37 mol%) were prepared using the melt-quenching method. The density of the glasses increases from 4.579 to 5.044 g/cm as a result of increase the PbO content. The radiation attenuation factors were experimentally determined at 0.059, 0.662, 1.173 and 1.333 MeV, using HPGe detector. The results indicate that increasing PbO content notably influences the mass attenuation coefficient and the effective atomic number. The tenth value layer (TVL) increased significantly with rising energy levels. For the glass sample containing 31 mol% PbO₂, the TVL increased from 0.177 cm at 0.059 MeV to 5.325 cm at 0.662 MeV, and to 9.094 cm at 1.333 MeV. Similarly, for the glass with 37 mol% PbO₂, the TVL increased from 0.146 cm at 0.059 MeV to 4.733 cm at 0.662 MeV, and to 8.231 cm at 1.333 MeV. The results also showed that PbO₂ has an inverse effect on the TVL, where adding more PbO₂ leads to a decrease in the TVL. At 0.662 MeV, increasing the PbO₂ content from 31 to 37 mol% reduces the TVL by approximately 11.12%. The transmission factor (TF) for the glass with a thickness of 2 cm was investigated, and results showed that the TF is nearly 0 at 0.059 MeV, indicating that the glass provides complete shielding at this low energy. The TF increases with rising energy, reaching 37.8-42.11% at 0.662 MeV, indicating that more photons penetrate the glass as the energy increases.
在本研究中,研究了将PbO融入硼硅酸盐玻璃体系以增强辐射屏蔽性能。采用熔融淬火法制备了几种PbO浓度不同(31、33、35和37 mol%)的玻璃。由于PbO含量增加,玻璃的密度从4.579 g/cm增加到5.044 g/cm。使用HPGe探测器在0.059、0.662、1.173和1.333 MeV下通过实验测定了辐射衰减因子。结果表明,增加PbO含量对质量衰减系数和有效原子序数有显著影响。第十值层(TVL)随着能级的升高而显著增加。对于含有31 mol% PbO₂的玻璃样品,TVL从0.059 MeV时的0.177 cm增加到0.662 MeV时的5.325 cm,以及1.333 MeV时的9.094 cm。同样,对于含有37 mol% PbO₂的玻璃,TVL从0.059 MeV时的0.146 cm增加到0.662 MeV时的4.733 cm,以及1.333 MeV时的8.231 cm。结果还表明,PbO₂对TVL有相反的影响,即添加更多的PbO₂会导致TVL降低。在0.662 MeV时,将PbO₂含量从31 mol%增加到37 mol%会使TVL降低约11.12%。研究了厚度为2 cm的玻璃的传输因子(TF),结果表明,在0.059 MeV时TF几乎为0,表明该玻璃在这种低能量下提供了完全屏蔽。TF随着能量的升高而增加,在0.662 MeV时达到37.8 - 42.11%,表明随着能量增加,更多的光子穿透玻璃。