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关于NiO(111)/Fe(110)双层膜中自旋重取向转变热滞现象的本质

On the nature of spin reorientation transition thermal hysteresis in NiO(111)/Fe(110) bilayers.

作者信息

Świerkosz E, Kwiatkowski A, Szpytma M, Janus W, Zając M, Dróżdż P, Oleś E, Kozioł-Rachwał A, Ślęzak T, Ślęzak M

机构信息

AGH University of Krakow, Kraków, Poland.

Elettra-Sincrotrone Trieste S.C.p.A, Basovizza, Trieste, Italy.

出版信息

Sci Rep. 2025 Jul 1;15(1):22267. doi: 10.1038/s41598-025-07541-1.

Abstract

We report on temperature-driven in-plane 90° magnetization switching in NiO(111)/Fe(110) bilayer epitaxially grown on a W(110) single crystal, investigated using magneto-optical Kerr effect and X-ray magnetic circular and linear dichroism measurements. As the temperature varies, an abrupt switching of the easy axis between the in-plane Fe[001] and Fe[Formula: see text] crystallographic directions is observed. In the temperature range of approximately 210-285 K, a thermal hysteresis region appears, where two energy minima coexist at a given temperature. Our experimental findings are supported by phenomenological modeling. Simulations incorporating temperature-dependent anisotropy constants successfully reproduce the key features of the observed phenomenon, most notably the temperature-driven hysteresis of ferromagnetic magnetization switching. The spin reorientation transition in both exchange-coupled ferromagnetic and antiferromagnetic layers is driven by the interplay between magnetocrystalline and interfacial magnetic anisotropies in the ferromagnet, which stabilizes specific magnetization orientation at given temperature.

摘要

我们报道了在W(110)单晶上外延生长的NiO(111)/Fe(110)双层膜中温度驱动的面内90°磁化翻转,通过磁光克尔效应以及X射线磁圆二色性和线性二色性测量进行了研究。随着温度变化,观察到易轴在面内Fe[001]和Fe[具体公式]晶体学方向之间发生突然翻转。在大约210 - 285 K的温度范围内,出现了一个热滞回区域,在给定温度下存在两个能量极小值。我们的实验结果得到了唯象模型的支持。纳入温度相关各向异性常数的模拟成功再现了所观察现象的关键特征,最显著的是铁磁磁化翻转的温度驱动滞回。在交换耦合的铁磁层和反铁磁层中的自旋重取向转变是由铁磁体中磁晶各向异性和界面磁各向异性之间的相互作用驱动的,这在给定温度下稳定了特定的磁化取向。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3626/12214746/4f1cd0064e3e/41598_2025_7541_Fig1_HTML.jpg

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