Barrat J L, Berthier L
Département de Physique des Matériaux, Université Claude Bernard and CNRS, Villeurbanne, France.
Phys Rev E Stat Nonlin Soft Matter Phys. 2001 Jan;63(1 Pt 1):012503. doi: 10.1103/PhysRevE.63.012503. Epub 2000 Dec 27.
In a fluid out of equilibrium, the fluctuation-dissipation theorem (FDT) is usually violated. Using molecular dynamics simulations, we study in detail the relationship between correlation and response functions in a fluid driven into a stationary nonequilibrium state. Both the high temperature fluid state and the low temperature glassy state are investigated. In the glassy state, the violation of the FDT is similar to the one observed previously in an aging system in the absence of external drive. In the fluid state, violations of the FDT appear only when the fluid is driven beyond the linear response regime, and are then similar to those observed in the glassy state. These results are consistent with the picture obtained earlier from theoretical studies of driven mean-field disordered models, confirming the similarity between these models and simple glassy systems.
在非平衡流体中,涨落耗散定理(FDT)通常不成立。我们使用分子动力学模拟,详细研究了被驱动到稳态非平衡态的流体中关联函数和响应函数之间的关系。我们研究了高温流体态和低温玻璃态。在玻璃态中,FDT的不成立与之前在无外部驱动的老化系统中观察到的情况类似。在流体态中,只有当流体被驱动到超出线性响应区域时,FDT才会不成立,且此时与在玻璃态中观察到的情况类似。这些结果与早期从驱动平均场无序模型的理论研究中得到的图像一致,证实了这些模型与简单玻璃态系统之间的相似性。