Gertler Alan W, Gillies John A, Pierson William R, Rogers C Fred, Sagebiel John C, Abu-Allaban Mahmoud, Coulombe William, Tarnay Leland, Cahill Thomas A
Division of Atmospheric Sciences, Desert Research Institute, Reno, NV 89512, USA.
Res Rep Health Eff Inst. 2002 Jan(107):5-56; discussion 79-92.
Recent studies have linked atmospheric particulate matter with human health problems. In many urban areas, mobile sources are a major source of particulate matter (PM) and the dominant source of fine particles or PM2.5 (PM smaller than 2.5 pm in aerodynamic diameter). Dynamometer studies have implicated diesel engines as being a significant source of ultrafine particles (< 0.1 microm), which may also exhibit deleterious health impacts. In addition to direct tailpipe emissions, mobile sources contribute to ambient particulate levels by brake and tire wear and by resuspension of particles from pavement. Information about particle emission rates, size distributions, and chemical composition from in-use light-duty (LD) and heavy-duty (HD) vehicles is scarce, especially under real-world operating conditions. To characterize particulate emissions from a limited set of in-use vehicles, we studied on-road emissions from vehicles operating under hot-stabilized conditions, at relatively constant speed, in the Tuscarora Mountain Tunnel along the Pennsylvania Turnpike from May 18 through 23, 1999. There were five specific aims of the study. (1) obtain chemically speciated diesel profiles for the source apportionment of diesel versus other ambient constituents in the air and to determine the chemical species present in real-world diesel emissions; (2) measure particle number and size distribution of chemically speciated particles in the atmosphere; (3) identify, by reference to data in years past, how much change has occurred in diesel exhaust particulate mass; (4) measure particulate emissions from LD gasoline vehicles to determine their contribution to the observed particle levels compared to diesels; and (5) determine changes over time in gas phase emissions by comparing our results with those of previous studies. Comparing the results of this study with our 1992 results, we found that emissions of C8 to C20 hydrocarbons, carbon monoxide (CO), and carbon dioxide (CO2) from HD diesel emissions substantially decreased over the seven-year period. Particulate mass emissions showed a similar trend. Considering a 25-year period, we observed a continued downward trend in HD particulate emissions from approximately 1,100 mg/km in 1974 to 132 mg/km (reported as PM2.5) in this study. The LD particle emission factor was considerably less than the HD value, but given the large fraction of LD vehicles, emissions from this source cannot be ignored. Results of the current study also indicate that both HD and LD vehicles emit ultrafine particles and that these particles are preserved under real-world dilution conditions. Particle number distributions were dominated by ultrafine particles with count mean diameters of 17 to 13 nm depending on fleet composition. These particles appear to be primarily composed of sulfur, indicative of sulfuric acid emission and nucleation. Comparing the 1992 and 1999 HD emission rates, we observed a 48% increase in the NOx/CO2 emissions ratio. This finding supports the assumption that many new-technology diesel engines conserve fuel but increase NOx emissions.
近期研究已将大气颗粒物与人类健康问题联系起来。在许多城市地区,移动源是颗粒物(PM)的主要来源,也是细颗粒物或PM2.5(空气动力学直径小于2.5微米的颗粒物)的主要来源。底盘测功机研究表明,柴油发动机是超细颗粒物(<0.1微米)的重要来源,这些超细颗粒物也可能对健康产生有害影响。除了直接的尾气排放外,移动源还通过制动和轮胎磨损以及路面颗粒物的再悬浮增加了环境颗粒物水平。关于在用轻型(LD)和重型(HD)车辆的颗粒物排放率、粒径分布和化学成分的信息很少,尤其是在实际运行条件下。为了表征有限数量的在用车辆的颗粒物排放情况,我们于1999年5月18日至23日在宾夕法尼亚收费公路沿线的图斯卡罗拉山隧道中,对在热稳定条件下以相对恒定速度行驶的车辆进行了道路排放研究。该研究有五个具体目标。(1)获取化学特征化的柴油排放概况,用于柴油与空气中其他环境成分的源解析,并确定实际柴油排放中存在的化学物质;(2)测量大气中化学特征化颗粒物的数量和粒径分布;(3)参考过去几年的数据,确定柴油尾气颗粒物质量发生了多大变化;(4)测量轻型汽油车的颗粒物排放,以确定其与柴油相比对观测到的颗粒物水平的贡献;(5)通过将我们的结果与以前的研究结果进行比较,确定气相排放随时间的变化。将本研究结果与我们1992年的结果进行比较,我们发现,在这七年期间,重型柴油排放中的C8至C20碳氢化合物、一氧化碳(CO)和二氧化碳(CO2)排放量大幅下降。颗粒物质量排放也呈现出类似趋势。考虑到25年的时间段,我们观察到重型颗粒物排放持续下降,从1974年的约1100毫克/公里降至本研究中的132毫克/公里(报告为PM2.5)。轻型颗粒物排放因子远低于重型排放因子,但鉴于轻型车辆数量众多,该来源的排放不容忽视。当前研究结果还表明,重型和轻型车辆都会排放超细颗粒物,并且这些颗粒物在实际稀释条件下得以保留。粒径分布以超细颗粒物为主,根据车队构成,计数平均直径在17至13纳米之间。这些颗粒物似乎主要由硫组成,表明存在硫酸排放和成核现象。比较1992年和1999年的重型排放率,我们发现氮氧化物/二氧化碳排放比增加了48%。这一发现支持了许多新技术柴油发动机节省燃料但增加氮氧化物排放的假设。