Edwards Boyd F
Department of Physics, West Virginia University, Morgantown 26506-6315, USA.
Phys Rev Lett. 2002 Sep 2;89(10):104501. doi: 10.1103/PhysRevLett.89.104501. Epub 2002 Aug 16.
Poiseuille flow between parallel plates alters the shapes and velocities of chemical reaction fronts. In the narrow-gap limit, the cubic reaction-diffusion-advection equation predicts a front-velocity correction equal to the gap-averaged fluid velocity epsilon. In the singular wide-gap limit, the correction equals the midgap fluid velocity 3epsilon/2 when the flow is in the direction of propagation of the reaction front, and equals zero for adverse flow of any amplitude for which the front has a midgap cusp. Stationary fronts are possible only for adverse flow and finite gaps. Experiments are suggested.
平行板间的泊肃叶流动会改变化学反应前沿的形状和速度。在窄间隙极限情况下,三次反应 - 扩散 - 平流方程预测前沿速度修正量等于间隙平均流体速度ε。在奇异的宽间隙极限情况下,当流动方向与反应前沿的传播方向一致时,修正量等于间隙中部流体速度3ε/2;而对于前沿在间隙中部有尖点的任何幅度的逆流,修正量都等于零。仅在逆流和有限间隙情况下才可能存在静止前沿。建议开展相关实验。