Franchi Paola, Lucarini Marco, Pedrielli Pamela, Pedulli Gian Franco
Dipartimento di Chimica Organica A. Mangini Università di Bologna Via S. Donato 15, 40127 Bologna, Italy.
Chemphyschem. 2002 Sep 16;3(9):789-93. doi: 10.1002/1439-7641(20020916)3:9<789::AID-CPHC789>3.0.CO;2-Z.
The equilibrium constants for the formation of hydrogen-bonded complexes with phenol, benzyl alcohol and diphenyl amine of a persistent nitroxide radical (TEMPO) have been measured for the first time by IR spectroscopy in solution. By making use of the data obtained with IR measurements it was possible to quantitatively determine the effect of hydrogen bonding on the nitrogen hyperfine-splitting constant. On this basis it is shown that EPR spectroscopy can be used as an alternative to IR spectroscopy for the determination of the thermodynamic parameters of hydrogen bond formation with nitroxides by following the dependence of the experimental EPR nitrogen hyperfine splitting of these radicals upon changing the nature of the solvent. The experimental data obtained from both IR and EPR spectroscopy indicate that nitroxides are versatile hydrogen bond acceptors giving hydrogen bonds of strength similar to that of ethers or esters. The corresponding Abraham's beta 2H values have been determined as 0.46.
首次通过溶液中的红外光谱法测量了持久性氮氧自由基(TEMPO)与苯酚、苯甲醇和二苯胺形成氢键复合物的平衡常数。利用红外测量获得的数据,可以定量确定氢键对氮超精细分裂常数的影响。在此基础上表明,通过跟踪这些自由基的实验EPR氮超精细分裂随溶剂性质变化的依赖性,EPR光谱法可作为红外光谱法的替代方法,用于测定与氮氧化物形成氢键的热力学参数。从红外光谱和EPR光谱获得的实验数据表明,氮氧化物是通用的氢键受体,形成的氢键强度与醚或酯的相似。相应的亚伯拉罕β2H值已确定为0.46。