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氧化银超分辨率近场结构中的光学跃迁过程。

Optical transition process in AgOx super-resolution near-field structure.

作者信息

Ho F H, Lin W Y, Chang H H, Wang P, Tsai D P

机构信息

Department of Physics, National Taiwan University, Taipei, Taiwan 10617, Republic of China.

出版信息

J Microsc. 2003 Mar;209(Pt 3):254-60. doi: 10.1046/j.1365-2818.2003.01121.x.

Abstract

A sandwiched 15 nm AgOx thin film of the super-resolution, near-field optical disk was studied using a confocal Z-scan system. Nonlinear optical properties of quartz glass/ZnS-SiO2 (170 nm)/AgOx (15 nm)/ZnS-SiO2 (40 nm) were measured using a Q-switch Nd : YAG pulse laser of wavelength 532 nm, pulse width 0.7 ns, and 15.79 kHz repetition rate. Transmittance and reflectance of the sandwiched AgOx thin film show important optical responses at the focused position of Z-scan. The dissociation processes of AgOx, recombination of the silver and oxygen, and the resonance of the localized surface plasmon of the nano-composites of the AgOx thin film are correlated to transmittance and reflectance at the focused position of the Z-scan for different input laser powers. An irreversible upper threshold intensity of 4.40 x 106 mW cm-2 at the focused position was found. A reversible working window of the focusing intensity between 1.86 x 106 and 4.40 x 106 mW cm-2 was measured with sandwiched AgOx thin film alone. The near-field interactions of the AgOx thin film and the recording layers of super-resolution near-field optical disk are also discussed.

摘要

利用共焦Z扫描系统对超分辨率近场光盘的15纳米夹心氧化银薄膜进行了研究。使用波长532纳米、脉冲宽度0.7纳秒、重复频率15.79千赫兹的调Q Nd:YAG脉冲激光测量了石英玻璃/ZnS-SiO2(170纳米)/AgOx(15纳米)/ZnS-SiO2(40纳米)的非线性光学特性。夹心氧化银薄膜的透过率和反射率在Z扫描的聚焦位置呈现出重要的光学响应。对于不同的输入激光功率,氧化银的离解过程、银与氧的复合以及氧化银薄膜纳米复合材料的局域表面等离子体共振与Z扫描聚焦位置处的透过率和反射率相关。在聚焦位置发现了4.40×10^6毫瓦/平方厘米的不可逆上阈值强度。仅使用夹心氧化银薄膜测量了1.86×10^6至4.40×10^6毫瓦/平方厘米之间的聚焦强度可逆工作窗口。还讨论了氧化银薄膜与超分辨率近场光盘记录层的近场相互作用。

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