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匈牙利奥伊考镇一家燃煤发电厂周围土壤中沉积的铀子体产生的室外伽马射线照射所致剂量增量的估算。

Estimate of the dose-increment due to outdoor exposure to gamma rays from uranium progeny deposited on the soil around a coal-fired power plant in Ajka Town, Hungary.

作者信息

Papp Z, Dezsö Z

机构信息

University of Debrecen, Faculty of Science-Institute of Nuclear Research, Department of Environmental Physics, PO Box 51, Debrecen 4001, Hungary.

出版信息

Health Phys. 2003 Jun;84(6):709-17. doi: 10.1097/00004032-200306000-00003.

Abstract

Brown coal unusually rich in uranium is burnt in a coal-fired power plant that lies inside the confines of a small industrial town named Ajka, Hungary, and has been operational since 1943. The 238U (226Ra) activity discharged to the atmosphere per unit electrical energy produced was about 330-400 GBq (GW y)(-1), which is 66-80 times more than that was estimated by UNSCEAR (1988) as a characteristic value for old type coal-fired power plants [5 GBq (GW y)(-1)]. The objective of this study was the experimentally established assessment of the artificial increment in the dose from external exposure to gamma rays of terrestrial radionuclides outdoors. Soil samples were collected in and near Ajka from 81 locations. The samples were investigated by Ge(Li) gamma spectrometry. Considerably elevated concentrations of uranium and its progeny have been measured in most of the samples that were collected near to the plant. Concentrations of 238U and 226Ra in the top (0-5 cm depth) layer of undisturbed soil at public areas inside town were 4.7 times higher, on average, than those in the uncontaminated deeper layers. Dose rate in air (air kerma) from external exposure to terrestrial gamma rays outdoors at a height of 1 m and effective doses were estimated from the measured activity concentrations using some relevant literature data. The estimated artificial increment in the dose rate in air was, on average, 32.8, 10.3, and 102.1 nGy h(-1) at public areas, vegetable gardens, and backyards, respectively. The mean artificial increment in the annual per caput effective dose from external exposure to terrestrial radionuclides outdoors is 21.8 microSv y(-1). The collective dose commitment per unit energy generated from outdoor exposure to the deposited uranium progeny is about 8.0-9.1 person Sv (GW y)(-1), which is 67-76 times more than that evaluated by UNSCEAR (1988) for a typical "old" coal-fired power plant [0.12 person Sv (GW y)(-1)]. Ajka is a suitable place for studying the dosimetric consequences of the utilization of coal for energy production experimentally.

摘要

在匈牙利一个名为奥伊考的小工业城镇范围内,有一座燃煤发电厂,该厂燃烧的褐煤中铀含量异常丰富,自1943年以来一直在运行。每产生单位电能排放到大气中的238U(226Ra)活度约为330 - 400 GBq(GW·y)(-1),这比联合国原子辐射效应科学委员会(1988年)估计的老式燃煤发电厂特征值[5 GBq(GW·y)(-1)]高出66 - 80倍。本研究的目的是通过实验确定室外陆地放射性核素伽马射线外照射剂量的人为增量。在奥伊考及其附近的81个地点采集了土壤样本。样本通过锗(锂)伽马能谱法进行检测。在靠近该厂采集的大多数样本中,铀及其子体的浓度都显著升高。城镇内公共区域未受扰动土壤表层(0 - 5厘米深度)的238U和226Ra浓度平均比未受污染的深层高出4.7倍。利用一些相关文献数据,根据测量的活度浓度估算了室外1米高度处陆地伽马射线外照射的空气剂量率(空气比释动能)和有效剂量。在公共区域、菜园和后院,估算的空气剂量率人为增量平均分别为32.8、10.3和102.1 nGy·h(-1)。室外陆地放射性核素外照射的人均年有效剂量人为增量平均值为21.8 μSv·y(-1)。室外暴露于沉降的铀子体产生的单位能量集体剂量承诺约为8.0 - 9.1人·Sv(GW·y)(-1),这比联合国原子辐射效应科学委员会(1988年)对典型“老式”燃煤发电厂评估的结果[0.12人·Sv(GW·y)(-1)]高出67 - 76倍。奥伊考是通过实验研究利用煤炭进行能源生产的剂量学后果的合适场所。

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