Vinage I, von Rohr Ph R
Institute of Process Engineering, ETH Zurich, Sonneggstrasse 3, 8092 Zurich, Switzerland.
Bioprocess Biosyst Eng. 2003 Nov;26(1):75-82. doi: 10.1007/s00449-003-0333-1. Epub 2003 Sep 19.
In the first part of this paper, we introduced a modified rotating biological contactor (RBC) for the biological treatment of waste gas, and demonstrated its feasibility by applying the process to the biodegradation of toluene in a 91-liter reactor containing 20 biofilm support discs with a diameter of 40 cm [1]. We showed that the proposed system allows the unlimited growth of the biofilm to be suppressed, hence eliminating the risk of clogging associated with other biological waste gas treatment systems. Furthermore, we observed stationary long-term performance for more than one year under typical standard operating conditions. In this part of our work, we investigate experimentally the influence of the main process parameters, i.e., gas flow rate, inlet gas concentration, and rotational speed of the biofilm supports on process performance for the same system. Experimental results indicate that the modified RBC system is mass transfer limited for toluene loadings below 150 g/m(3)h, whereas at higher inlet concentrations of the pollutant, it becomes limited by the biodegradation reaction inside the biofilm. Surprisingly, the disc rotational speed is found to have no major effect on process performance for the system under investigation. A time-independent mathematical model of the process is also presented, and predictions are compared with experimental degradation data. In the range of the investigation process parameters, good agreement between the experimental data and simulation results is obtained.
在本文的第一部分,我们介绍了一种用于废气生物处理的改良型旋转生物接触器(RBC),并通过将该工艺应用于在一个装有20个直径为40厘米的生物膜支撑盘的91升反应器中甲苯的生物降解,证明了其可行性[1]。我们表明,所提出的系统能够抑制生物膜的无限制生长,从而消除了与其他生物废气处理系统相关的堵塞风险。此外,我们观察到在典型的标准操作条件下,该系统能够保持一年以上的稳定长期性能。在我们工作的这一部分中,我们对同一系统实验研究了主要工艺参数,即气体流速、进气浓度和生物膜支撑盘的转速对工艺性能的影响。实验结果表明,对于甲苯负荷低于150克/立方米·小时的情况,改良型RBC系统受传质限制,而在污染物进气浓度较高时,它受生物膜内生物降解反应的限制。令人惊讶的是,发现盘的转速对所研究系统的工艺性能没有重大影响。还提出了该工艺的一个与时间无关的数学模型,并将预测结果与实验降解数据进行了比较。在研究的工艺参数范围内,实验数据与模拟结果之间取得了良好的一致性。