Oh Sung-Nam, Sohn Byung-Ju, Lee Sang-Sam
National Research Laboratory, Meteorological Research Institute, KMA, Seoul, Korea.
Environ Monit Assess. 2004 Mar;92(1-3):95-115. doi: 10.1023/b:emas.0000014511.81178.3f.
The radiative properties of atmospheric aerosols are determined by their masses, chemical characteristics, and optical properties, such as aerosol optical depth (AOD), Angström parameter (alpha) and single scattering albedo (SSA). In particular, the aerosol optical properties determine the surface temperature perturbation that may give some information in understanding regional atmospheric radiative forcing. To understand the radiative forcing and regional source of an aerosol, the present study focused on the analysis of the aerosol optical properties based on two different observations in the spring season, during the special Asian dust storm period. The Korean Global Atmosphere Watch Observatory (KGAWO), at Anmyeon Island, and the ACE-Asia super-site, at Gosan, Jeju Island, have measured radiations and aerosols since 2000. The sites are located in the mid-west and south of the Korean peninsula, which are strongly affected by the Asian dust coming from China every spring. The aerosol optical properties, measured by ground-based sun and sky radiometers, over both sites were analyzed to gain an understanding of the radiation and climate properties. The probability distributions of the aerosol optical depths were rather narrow, with a modal value of approximately 0.38 at both sites during 2001 and 2002. The Angström parameter frequency distributions showed two peaks at Anmyeon GAW, but only one peak at the Jeju ACE-Asia super site. One peak, around 0.63, characterizes the situation of a day having Asian dust, the second peak, around 1.13, corresponded to the relatively dust-free cases. The correlation between the aerosol optical depth and the Angström exponents resulted in a wide range of the Angström parameter, alpha, over a wide range of optical depths at Anmyeon, whereas a narrow range of alpha, with moderate to low values for the AOD at Jeju. Under dust free conditions the single scattering albedo (SSA) decreased with wavelength, while in the presence of Asian dust, the SSA either stayed neutral, or increased slightly with wavelength at Anmyeon, and showed higher value than Jeju. The change in the surface temperature was highly correlated with increases in the aerosol optical depth at Anmyeon to a greater extent than at Jeju.
大气气溶胶的辐射特性由其质量、化学特性以及光学特性决定,如气溶胶光学厚度(AOD)、Ångström参数(α)和单次散射反照率(SSA)。特别是,气溶胶光学特性决定了地表温度扰动,这可能为理解区域大气辐射强迫提供一些信息。为了理解气溶胶的辐射强迫和区域来源,本研究重点基于春季特殊亚洲沙尘暴期间的两种不同观测数据,对气溶胶光学特性进行分析。位于安眠岛的韩国全球大气观测站(KGAWO)和济州岛高山市的ACE-亚洲超级站点自2000年以来一直在测量辐射和气溶胶。这些站点位于朝鲜半岛中西部和南部,每年春天都受到来自中国的亚洲沙尘的强烈影响。通过地基太阳和天空辐射计测量的两个站点的气溶胶光学特性,以了解辐射和气候特性。2001年和2002年期间,两个站点的气溶胶光学厚度概率分布相当窄,模态值约为0.38。Ångström参数频率分布在安眠全球大气观测站显示出两个峰值,但在济州岛ACE-亚洲超级站点仅显示一个峰值。一个峰值约为0.63,表征有亚洲沙尘的日子的情况,第二个峰值约为1.13,对应相对无沙尘的情况。在安眠岛,气溶胶光学厚度与Ångström指数之间的相关性导致在较宽的光学厚度范围内,Ångström参数α的范围很广,而在济州岛,α的范围较窄,AOD值为中低值。在无沙尘条件下,单次散射反照率(SSA)随波长降低,而在有亚洲沙尘的情况下,在安眠岛SSA要么保持中性,要么随波长略有增加,且显示出比济州岛更高的值。与济州岛相比,安眠岛地表温度的变化在更大程度上与气溶胶光学厚度的增加高度相关。