Duran E B, Povinec P P, Fowler S W, Airey P L, Hong G H
Philippine Nuclear Research Institute, Commonwealth Avenue, Diliman, Quezon City, Philippines.
J Environ Radioact. 2004;76(1-2):139-60. doi: 10.1016/j.jenvrad.2004.03.023.
137Cs and (239+240)Pu data in seawater, sediment and biota from the regional seas of Asia-Pacific extending from 50 degrees N to 60 degrees S latitude and 60 degrees E to 180 degrees E longitude based on the Asia-Pacific Marine Radioactivity Database (ASPAMARD) are presented and discussed. 137Cs levels in surface seawater have been declining to its present median value of about 3 Bq/m3 due mainly to radioactive decay, transport processes, and the absence of new significant inputs. (239+240)Pu levels in surface seawater are much lower, with a median of about 6 mBq/m3. (239+240)Pu appears to be partly scavenged by particles and is therefore more readily transported down the water column. As with seawater, (239+240)Pu concentrations are lower than 137Cs in surface sediment. The median 137Cs concentration in surface sediment is 1.4 Bq/kg dry, while that of (239+240)Pu is only 0.2 Bq/kg dry. The vertical profiles of both 137Cs and (239+240)Pu in the sediment column of coastal areas are different from deep seas which can be attributed to the higher sedimentation rates and additional contribution of run-offs from terrestrial catchment areas in the coastal zone. Comparable data for biota are far less extensive than those for seawater and sediment. The median 137Cs concentration in fish (0.2 Bq/kg wet) is higher than in crustaceans (0.1 Bq/kg wet) or mollusks (0.1 Bq/kg wet). Benchmark values (as of 2001) for 137Cs and (239+240)Pu concentrations in seawater, sediment and biota are established to serve as reference values against which the impact of future anthropogenic inputs can be assessed. ASPAMARD represents one of the most comprehensive compilations of available data on 137Cs and (239+240)Pu in particular, and other anthropogenic as well as natural radionuclides in seawater, sediment and biota from the Asia-Pacific regional seas.
基于亚太海洋放射性数据库(ASPAMARD),给出并讨论了从北纬50度至南纬60度、东经60度至180度的亚太区域海域海水、沉积物和生物群中的137铯和(239+240)钚数据。表层海水中的137铯水平一直在下降,目前的中值约为3贝可勒尔/立方米,这主要归因于放射性衰变、迁移过程以及没有新的重大输入。表层海水中(239+240)钚的水平要低得多,中值约为6毫贝可勒尔/立方米。(239+240)钚似乎部分被颗粒清除,因此更容易在水柱中向下迁移。与海水一样,表层沉积物中(239+240)钚的浓度低于137铯。表层沉积物中137铯的中值浓度为1.4贝可勒尔/千克干重,而(239+240)钚仅为0.2贝可勒尔/千克干重。沿海地区沉积物柱中137铯和(239+240)钚的垂直分布与深海不同,这可归因于较高的沉积速率以及沿海地区陆地集水区径流的额外贡献。生物群的可比数据远不如海水和沉积物的数据广泛。鱼类中137铯的中值浓度(0.2贝可勒尔/千克湿重)高于甲壳类动物(0.1贝可勒尔/千克湿重)或软体动物(0.1贝可勒尔/千克湿重)。确定了海水、沉积物和生物群中137铯和(239+240)钚浓度的基准值(截至2001年),作为评估未来人为输入影响的参考值。ASPAMARD是关于137铯和(239+240)钚,特别是亚太区域海域海水、沉积物和生物群中其他人为和天然放射性核素的现有数据最全面的汇编之一。