Zhao Fu, Landis Heather R, Skerlos Steven J
Environmental and Sustainable Technologies Laboratory, Department of Mechanical Engineering, University of Michigan at Ann Arbor, Ann Arbor, Michigan 48109-2125, USA.
Environ Sci Technol. 2005 Jan 1;39(1):239-47. doi: 10.1021/es035228b.
A methodology for producing a pore-scale, 3D computational model of porous filter permeability is developed that is based on the analysis of 2D images of the filter matrix and first principles. The computationally reconstructed porous filter model retains statistical details of porosity and the spatial correlations of porosity within the filter and can be used to calculate permeability for either isotropic or 1D anisotropic porous filters. In the isotropic case, validation of the methodology was conducted using 0.2 and 0.8 microm ceramic membrane filters,forwhich it is shown that the image-based computational models provide a viable statistical reproduction of actual porosity characteristics. It is also shown that these models can predict water flux directly from first principles with deviations from experimental measurements in the range of experimental error. In the anisotropic case, validation of the methodology was conducted using a natural river sand filter. For this case, it is shown that the methodology yields predictions of filtration velocity that are similar or better than predictions offered by existing filtration models. It was found for the sand filter that the deviation between observation and prediction was mostly due to swelling during the preparation of the sand filter for imaging and can be reduced significantly using alternative methods reported in the literature. On the basis of these results, it is concluded that the computational reconstruction methodology is valid for porous filter modeling, and given that it captures pore-scale details, it has potential application to the investigation of permeability decline underthe influence of pore-scale fouling mechanisms.
基于对过滤介质二维图像的分析和第一性原理,开发了一种用于生成孔隙尺度的多孔过滤器渗透率三维计算模型的方法。通过计算重建的多孔过滤器模型保留了孔隙率的统计细节以及过滤器内孔隙率的空间相关性,可用于计算各向同性或一维各向异性多孔过滤器的渗透率。在各向同性情况下,使用0.2微米和0.8微米的陶瓷膜过滤器对该方法进行了验证,结果表明基于图像的计算模型能够对实际孔隙率特征进行有效的统计再现。研究还表明,这些模型可以直接根据第一性原理预测水通量,与实验测量值的偏差在实验误差范围内。在各向异性情况下,使用天然河砂过滤器对该方法进行了验证。对于这种情况,结果表明该方法得出的过滤速度预测值与现有过滤模型提供的预测值相似或更好。对于砂滤器,发现观测值与预测值之间的偏差主要是由于在制备用于成像的砂滤器过程中发生了膨胀,使用文献中报道的替代方法可以显著降低这种偏差。基于这些结果,可以得出结论,计算重建方法对于多孔过滤器建模是有效的,并且由于它能够捕捉孔隙尺度的细节,因此在研究孔隙尺度污垢机制影响下的渗透率下降方面具有潜在的应用价值。