Sandberg Eric M, Ma Xianyue, He Kai, Frank Stuart J, Ostrov David A, Sayeski Peter P
Department of Physiology and Functional Genomics, University of Florida College of Medicine, Gainesville, Florida 32610, USA.
J Med Chem. 2005 Apr 7;48(7):2526-33. doi: 10.1021/jm049470k.
The commercially available Jak2 inhibitor, alpha-cyano-3,4-dihydroxy-N-benzylcinnamide (AG490), has been used extensively to study Jak2 kinase function. While alpha-cyano-3,4-dihydroxy-N-benzylcinnamide is a potent Jak2 inhibitor, it can inhibit a number of other kinase signaling pathways as well. To circumvent this problem, we sought to identify novel small molecule inhibitors of Jak2 tyrosine kinase activity. For this, we constructed a homology model of the Jak2 kinase domain and identified solvent accessible pockets on the surface of the structure. Using the DOCK program, we tested 6451 compounds of known chemical structure in silico for their ability to interact with a pocket positioned adjacent to the activation loop. We attained the top seven scoring compounds from the National Cancer Institute and tested their ability to inhibit Jak2 autophosphorylation in vitro. Using Western blot analysis, we found that one of the compounds, 1,2,3,4,5,6-hexabromocyclohexane, was able to potently, and directly, inhibit Jak2 autophosphorylation. Characterization of this compound revealed that it inhibits Jak2 tyrosine autophosphorylation in both a time- and concentration-dependent manner. It greatly reduced growth hormone-mediated Jak2 autophosphorylation but did not block autophosphorylation of the epidermal growth factor receptor. Furthermore, doses as high as 100 muM were not toxic to cells as measured by their ability to exclude propidium iodide. As such, we believe that this compound could serve as a lead compound for a new generation of Jak2 inhibitors and, perhaps, be useful in elucidating the mechanisms of Jak2 kinase function.
市售的Jak2抑制剂α-氰基-3,4-二羟基-N-苄基肉桂酰胺(AG490)已被广泛用于研究Jak2激酶功能。虽然α-氰基-3,4-二羟基-N-苄基肉桂酰胺是一种有效的Jak2抑制剂,但它也能抑制许多其他激酶信号通路。为了解决这个问题,我们试图鉴定Jak2酪氨酸激酶活性的新型小分子抑制剂。为此,我们构建了Jak2激酶结构域的同源模型,并确定了该结构表面可及的溶剂口袋。使用DOCK程序,我们在计算机上测试了6451种已知化学结构的化合物与位于激活环附近口袋相互作用的能力。我们从美国国立癌症研究所获得了得分最高的七种化合物,并测试了它们在体外抑制Jak2自身磷酸化的能力。通过蛋白质印迹分析,我们发现其中一种化合物1,2,3,4,5,6-六溴环己烷能够有效且直接地抑制Jak2自身磷酸化。对该化合物的表征显示,它以时间和浓度依赖性方式抑制Jak2酪氨酸自身磷酸化。它极大地降低了生长激素介导的Jak2自身磷酸化,但并未阻断表皮生长因子受体的自身磷酸化。此外,高达100μM的剂量对细胞无毒,这通过它们排斥碘化丙啶的能力来衡量。因此,我们认为该化合物可以作为新一代Jak2抑制剂的先导化合物,并且可能有助于阐明Jak2激酶功能的机制。