Uddin M S, Hagiwara M, Baba M, Tarkanyi F, Ditroi F
Cyclotron and Radioisotope Center, Tohoku University, Aramaki, Aoba-ku, Sendai 980-8578, Japan.
Appl Radiat Isot. 2005 Sep;63(3):367-74. doi: 10.1016/j.apradiso.2005.04.006.
Proton-induced activation cross-sections were measured for the (89)Y(p,x)(89,88,86)Zr, (89)Y(p,x)(88,87,87 m,86)Y, (89)Y(p,x)(85,83,82)Sr and (89)Y(p,x)(84,83)Rb reactions by a stacked foil technique in the energy range 15-80 MeV which was covered by two separate measurements for 15-50 and 32-80 MeV energy range with 50 and 80 MeV incident protons. The differences between the results of two irradiations were found within 6% in the overlapping energy regions. The production yields for the long-lived products like (88)Zr, and (88)Y are significantly larger than that of (nat)Mo+p, (nat)Nb+p and (nat)Zr+p processes. The productions of the medical isotopes, (85)Sr and (83)Sr are also effective by Y+p process using an 80 MeV beam. Thick target integral yields were also deduced using the measured cross-sections. The (87)Y, (88)Y, (88)Zr and (89)Zr radionuclides have suitable yields and decay characteristics important for thin-layer activation (TLA) analysis.
采用叠层箔技术,在15 - 80 MeV能量范围内测量了质子诱发的(89)Y(p,x)(89,88,86)Zr、(89)Y(p,x)(88,87,87m,86)Y、(89)Y(p,x)(85,83,82)Sr和(89)Y(p,x)(84,83)Rb反应的活化截面。该能量范围通过对15 - 50 MeV和32 - 80 MeV能量范围进行两次单独测量覆盖,入射质子能量分别为50 MeV和80 MeV。在重叠能量区域内,两次辐照结果的差异在6%以内。(88)Zr和(88)Y等长寿命产物的产额明显高于(nat)Mo + p、(nat)Nb + p和(nat)Zr + p过程的产额。使用80 MeV束流的Y + p过程对医用同位素(85)Sr和(83)Sr的产生也很有效。还利用测量的截面推导了厚靶积分产额。(87)Y、(88)Y、(88)Zr和(89)Zr放射性核素具有适合薄层活化(TLA)分析的产额和衰变特性。