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通过K壳层X射线发射测量研究激光辐照氩团簇动力学。

Investigation of laser-irradiated Ar cluster dynamics from K-shell x-ray emission measurements.

作者信息

Dorchies F, Caillaud T, Blasco F, Bonté C, Jouin H, Micheau S, Pons B, Stevefelt J

机构信息

CELIA, UMR 5107, CNRS, CEA, Université Bordeaux I, 33405 Talence, France.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2005 Jun;71(6 Pt 2):066410. doi: 10.1103/PhysRevE.71.066410. Epub 2005 Jun 27.

Abstract

Intense (up to a few 10(17) W/ cm2) femtosecond (down to 40 fs) laser pulses are focused onto a partially clusterized argon gas jet. The target was previously characterized and optimized in order to get a homogeneous and dense jet of clusters with a well controlled size. The interaction leads to x-ray emission that is absolutely calibrated and spectrally resolved using a high resolution time-integrated spectrometer in the K-shell range (from 2.9 to 4.3 keV). X-ray spectra are investigated as a function of different laser temporal parameters such as the nanosecond prepulse contrast, the laser pulse duration, and the femtosecond delay between two different laser pulses. The cluster size ranges from 180 to 350 angstroms and irradiation by laser pulses with both linear and circular polarization is investigated. The experimental results are discussed in terms of the laser-cluster interaction dynamics. They are compared with the predictions of collision-dominated nanoplasma models. However, further interaction processes are required in order to explain the observed characteristic lines demonstrating highly charged ions up to Ar16+.

摘要

高强度(高达几×10¹⁷瓦/平方厘米)的飞秒(低至40飞秒)激光脉冲聚焦到部分团簇化的氩气喷流上。此前已对靶材进行了表征和优化,以获得尺寸可控的均匀且密集的团簇喷流。相互作用会产生X射线发射,使用高分辨率时间积分光谱仪在K壳层范围(2.9至4.3千电子伏特)内对其进行绝对校准和光谱分辨。研究了X射线光谱作为不同激光时间参数的函数,如纳秒预脉冲对比度、激光脉冲持续时间以及两个不同激光脉冲之间的飞秒延迟。团簇尺寸范围为180至350埃,并研究了线性和圆偏振激光脉冲的辐照情况。根据激光与团簇相互作用动力学对实验结果进行了讨论。将其与碰撞主导的纳米等离子体模型的预测结果进行了比较。然而,为了解释观察到的显示高达Ar¹⁶⁺的高电荷离子的特征谱线,还需要进一步的相互作用过程。

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