Honzatko Ales, Brichac Jiri, Murphy Tonya C, Reberg Alexander, Kubátová Alena, Smoliakova Irina P, Picklo Matthew J
Department of Pharmacology, Physiology, and Therapeutics, School of Medicine and Health Sciences, University of North Dakota, Grand Forks, ND 58202-9024, USA.
Free Radic Biol Med. 2005 Oct 1;39(7):913-24. doi: 10.1016/j.freeradbiomed.2005.05.010.
Trans-4-hydroxy-2-nonenal (HNE) is a product of lipid peroxidation with many cellular effects. HNE possesses a stereogenic center at the C4 carbon that influences the metabolism and alkylation targets of HNE. We tested the hypothesis that rat brain mitochondria metabolize HNE in an enantioselective manner after exposure to racemic HNE. The study of HNE chirality, however, is hindered by the lack of facile methods to chromatographically resolve (R)-HNE and (S)-HNE. We used a chiral hydrazine, (S)-carbidopa, as a derivatization reagent to form diastereomers with (R)-HNE and (S)-HNE that were separated by reverse-phase HPLC. After exposure to racemic HNE, rat brain mitochondria metabolized HNE enantioselectively with a higher rate of (R)-HNE metabolism. By using the purified enantiomers of HNE, we found that this enantioselective metabolism of HNE was the result of higher rates of enzymatic oxidation of (R)-HNE by aldehyde dehydrogenases compared to (S)-HNE. Conjugation of HNE to glutathione was a minor metabolic pathway and was not enantioselective. These studies demonstrate that the chirality of HNE affects its mitochondrial metabolism and potentially other processes in the central nervous system.
反式-4-羟基-2-壬烯醛(HNE)是脂质过氧化的产物,具有多种细胞效应。HNE在C4碳上有一个手性中心,该中心影响HNE的代谢和烷基化靶点。我们测试了以下假设:大鼠脑线粒体在暴露于外消旋HNE后以对映体选择性方式代谢HNE。然而,由于缺乏简便的色谱分离方法来分离(R)-HNE和(S)-HNE,HNE手性的研究受到了阻碍。我们使用手性肼(S)-卡比多巴作为衍生化试剂,与(R)-HNE和(S)-HNE形成非对映异构体,通过反相高效液相色谱进行分离。暴露于外消旋HNE后,大鼠脑线粒体以对映体选择性方式代谢HNE,(R)-HNE的代谢速率更高。通过使用纯化的HNE对映体,我们发现HNE的这种对映体选择性代谢是由于醛脱氢酶对(R)-HNE的酶促氧化速率高于(S)-HNE。HNE与谷胱甘肽的结合是一条次要的代谢途径,且没有对映体选择性。这些研究表明,HNE的手性影响其线粒体代谢,并可能影响中枢神经系统中的其他过程。