Hill J, Harris A W, Manning M, Chambers A, Swanton S W
UK Nirex Limited, Curie Avenue, Harwell, Didcot Oxfordshire, OX11 0RH, United Kingdom.
Waste Manag. 2006;26(7):758-68. doi: 10.1016/j.wasman.2006.01.022. Epub 2006 Mar 13.
The use of cement based materials will be widespread in the long-term management of radioactive materials in the United Kingdom. One of the applications could be the Nirex reference vault backfill (NRVB) as an engineered barrier within a deep geological repository. NRVB confers alkaline conditions, which would provide a robust chemical barrier through the control of the solubility of some key radionuclides, enhanced sorption and minimised corrosion of steel containers. An understanding of the dissolution of C-S-H gels in cement under the appropriate conditions (e.g., saline groundwaters) is necessary to demonstrate the expected evolution of the chemistry over time and to provide sufficient cement to buffer the porewater conditions for the required time. A programme of experimental work has been undertaken to investigate C-S-H gel dissolution behaviour in sodium chloride solutions and the effect of calcium/silicon ratio (C/S), temperature and cation type on this behaviour. Reductions in calcium concentration and pH values were observed with samples equilibrated at 45 degrees C compared to those prepared at 25 degrees C. The effect of salt cation type on salt-concentration dependence of the dissolution of C-S-H gels was investigated by the addition of lithium or potassium chloride in place of sodium chloride for gels with a C/S of 1.0 and 1.8. With a C/S of 1.0, similar increases in dissolved calcium concentration with increasing ionic strength were recorded for the different salts. However, at a C/S of 1.8, anomalously high calcium concentrations were observed in the presence of lithium.
在英国,水泥基材料在放射性材料的长期管理中将得到广泛应用。其中一个应用可能是作为深部地质处置库中的工程屏障的Nirex参考库回填材料(NRVB)。NRVB能营造碱性条件,通过控制某些关键放射性核素的溶解度、增强吸附作用以及使钢容器的腐蚀最小化,从而提供强大的化学屏障。了解在适当条件下(如含盐地下水)水泥中C-S-H凝胶的溶解情况,对于证明随着时间推移化学性质的预期演变以及提供足够的水泥以在所需时间内缓冲孔隙水条件是必要的。已开展了一项实验工作计划,以研究C-S-H凝胶在氯化钠溶液中的溶解行为以及钙/硅比(C/S)、温度和阳离子类型对该行为的影响。与在25摄氏度下制备的样品相比,在45摄氏度下平衡的样品中观察到钙浓度和pH值降低。通过添加氯化锂或氯化钾代替氯化钠,对C/S为1.0和1.8的凝胶研究了盐阳离子类型对C-S-H凝胶溶解的盐浓度依赖性的影响。对于C/S为1.0的情况,不同盐类随着离子强度增加溶解钙浓度有类似的增加。然而,在C/S为1.8时,在锂存在的情况下观察到异常高的钙浓度。