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距离和流量对大砾石柱中微球运移的影响

Distance and flow effects on microsphere transport in a large gravel column.

作者信息

Close Murray E, Pang Liping, Flintoft Mark J, Sinton Lester W

机构信息

Institute of Environmental Science & Research Ltd., P.O. Box 29181, Christchurch, New Zealand.

出版信息

J Environ Qual. 2006 Jul 6;35(4):1204-12. doi: 10.2134/jeq2005.0286. Print 2006 Jul-Aug.

Abstract

Consumption of microbially contaminated ground water can cause adverse health effects and the processes involved in pathogen transport in aquifers need to be understood. The influences of distance, flow velocity, and colloid size on colloid transport were examined in homogenous pea-gravel media using an 8-m column and three sizes (1, 5, and 10 microm) of microspheres. Experiments were conducted at three flow rates by simultaneously injecting microspheres with a conservative tracer, bromide. Observed concentrations were simulated with CXTFIT and analyzed with filtration theory. The results demonstrate that colloid concentration is strongly log-linearly related to transport distance (as suggested by filtration theory) in coarse gravels, similar to our previous field studies. In contrast, the log-linear relationship is often reported to be invalid in fine porous media. The observed log-linear relationship is possibly because straining is negligible in the coarse gravels investigated. This has implications in predicting setback distances for land disposal of effluent, and suggests that setback distances in gravel aquifers can be estimated using constant spatial removal rates (f). There was an inverse relationship between transport distance and colloidal concentration, but not with temporal attachment rate (katt) and collision coefficient (alpha). Increases in flow velocity result in increasing colloidal recovery, katt and alpha but decreasing f. Increases in sphere size result in decreasing colloidal recovery with increasing katt, f, alpha, and velocity enhancement. Diffusion is the dominant collision mechanism for 1-microm spheres (81-88%), while settling dominates for 5- and 10-microm spheres (> 87%), and interception is very small for all spheres investigated.

摘要

饮用受微生物污染的地下水会对健康产生不利影响,因此需要了解病原体在含水层中迁移的过程。使用一个8米长的柱子和三种尺寸(1、5和10微米)的微球,在均质豌豆砾石介质中研究了距离、流速和胶体尺寸对胶体迁移的影响。通过同时注入微球和保守示踪剂溴化物,在三种流速下进行了实验。用CXTFIT模拟观测浓度,并根据过滤理论进行分析。结果表明,在粗砾石中,胶体浓度与迁移距离呈强对数线性关系(如过滤理论所暗示),这与我们之前的现场研究类似。相比之下,对数线性关系在细孔隙介质中通常被认为是无效的。观察到的对数线性关系可能是因为在所研究的粗砾石中,过滤作用可以忽略不计。这对预测废水土地处置的退缩距离具有启示意义,并表明可以使用恒定的空间去除率(f)来估计砾石含水层中的退缩距离。迁移距离与胶体浓度呈反比关系,但与时间附着率(katt)和碰撞系数(alpha)无关。流速增加会导致胶体回收率、katt和alpha增加,但f降低。球体尺寸增加会导致胶体回收率降低,同时katt、f、alpha和速度增强增加。对于1微米的球体,扩散是主要的碰撞机制(81-88%),而对于5微米和10微米的球体,沉降占主导(>87%),对于所有研究的球体,拦截作用都非常小。

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