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超重元素中的核异构体作为通向稳定岛的垫脚石。

Nuclear isomers in superheavy elements as stepping stones towards the island of stability.

作者信息

Herzberg R-D, Greenlees P T, Butler P A, Jones G D, Venhart M, Darby I G, Eeckhaudt S, Eskola K, Grahn T, Gray-Jones C, Hessberger F P, Jones P, Julin R, Juutinen S, Ketelhut S, Korten W, Leino M, Leppänen A-P, Moon S, Nyman M, Page R D, Pakarinen J, Pritchard A, Rahkila P, Sarén J, Scholey C, Steer A, Sun Y, Theisen Ch, Uusitalo J

机构信息

Department of Physics, University of Liverpool, Liverpool L69 7ZE, UK.

出版信息

Nature. 2006 Aug 24;442(7105):896-9. doi: 10.1038/nature05069.

DOI:10.1038/nature05069
PMID:16929293
Abstract

A long-standing prediction of nuclear models is the emergence of a region of long-lived, or even stable, superheavy elements beyond the actinides. These nuclei owe their enhanced stability to closed shells in the structure of both protons and neutrons. However, theoretical approaches to date do not yield consistent predictions of the precise limits of the 'island of stability'; experimental studies are therefore crucial. The bulk of experimental effort so far has been focused on the direct creation of superheavy elements in heavy ion fusion reactions, leading to the production of elements up to proton number Z = 118 (refs 4, 5). Recently, it has become possible to make detailed spectroscopic studies of nuclei beyond fermium (Z = 100), with the aim of understanding the underlying single-particle structure of superheavy elements. Here we report such a study of the nobelium isotope 254No, with 102 protons and 152 neutrons--the heaviest nucleus studied in this manner to date. We find three excited structures, two of which are isomeric (metastable). One of these structures is firmly assigned to a two-proton excitation. These states are highly significant as their location is sensitive to single-particle levels above the gap in shell energies predicted at Z = 114, and thus provide a microscopic benchmark for nuclear models of the superheavy elements.

摘要

核模型的一个长期预测是,在锕系元素之后会出现一个长寿命甚至稳定的超重元素区域。这些原子核稳定性增强归因于质子和中子结构中的封闭壳层。然而,迄今为止的理论方法对于“稳定岛”的精确界限并未给出一致的预测;因此,实验研究至关重要。到目前为止,大部分实验工作都集中在通过重离子聚变反应直接产生超重元素,从而产生了质子数Z = 118以内的元素(参考文献4、5)。最近,对镄(Z = 100)之后的原子核进行详细光谱研究成为可能,目的是了解超重元素潜在的单粒子结构。在此,我们报告对锘同位素²⁵⁴No的此类研究,它有102个质子和152个中子,是迄今为止以这种方式研究的最重原子核。我们发现了三种激发结构,其中两种是同质异能的(亚稳态)。其中一种结构被明确归因为双质子激发。这些态非常重要,因为它们的位置对Z = 114时预测的壳层能量间隙之上的单粒子能级敏感,因此为超重元素的核模型提供了一个微观基准。

相似文献

1
Nuclear isomers in superheavy elements as stepping stones towards the island of stability.超重元素中的核异构体作为通向稳定岛的垫脚石。
Nature. 2006 Aug 24;442(7105):896-9. doi: 10.1038/nature05069.
2
Direct mapping of nuclear shell effects in the heaviest elements.直接映射最重元素中的核壳效应。
Science. 2012 Sep 7;337(6099):1207-10. doi: 10.1126/science.1225636. Epub 2012 Aug 9.
3
'Magic' nucleus 42Si.“神奇”的原子核42硅
Nature. 2005 Jun 16;435(7044):922-4. doi: 10.1038/nature03619.
4
Shape coexistence and triaxiality in the superheavy nuclei.超重核中的形状共存与三轴性
Nature. 2005 Feb 17;433(7027):705-9. doi: 10.1038/nature03336.
5
Chemistry of superheavy elements.超重元素的化学
Angew Chem Int Ed Engl. 2006 Jan 9;45(3):368-401. doi: 10.1002/anie.200461072.
6
Discovery of 40Mg and 42Al suggests neutron drip-line slant towards heavier isotopes.40Mg和42Al的发现表明中子滴线向较重同位素倾斜。
Nature. 2007 Oct 25;449(7165):1022-4. doi: 10.1038/nature06213.
7
Chemical characterization of element 112.第112号元素的化学特性
Nature. 2007 May 3;447(7140):72-5. doi: 10.1038/nature05761.
8
Shell-structure and pairing interaction in superheavy nuclei: rotational properties of the z=104 nucleus (256)rf.壳层结构和超重核中的配对相互作用:Z=104 核(256)rf 的转动性质。
Phys Rev Lett. 2012 Jul 6;109(1):012501. doi: 10.1103/PhysRevLett.109.012501. Epub 2012 Jul 3.
9
K isomers in 254No: probing single-particle energies and pairing strengths in the heaviest nuclei.254No中的K异构体:探索最重原子核中的单粒子能量和配对强度
Phys Rev Lett. 2006 Aug 25;97(8):082502. doi: 10.1103/PhysRevLett.97.082502. Epub 2006 Aug 22.
10
Mass and lifetime measurements of exotic nuclei in storage rings.储存环中奇异原子核的质量和寿命测量。
Mass Spectrom Rev. 2008 Sep-Oct;27(5):428-69. doi: 10.1002/mas.20173.

引用本文的文献

1
Direct mass measurements above uranium bridge the gap to the island of stability.直接测量铀桥上方的质量填补了稳定岛的空白。
Nature. 2010 Feb 11;463(7282):785-8. doi: 10.1038/nature08774.