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通过相干X射线散射研究层状相中的体涨落动力学。

Dynamics of bulk fluctuations in a lamellar phase studied by coherent x-ray scattering.

作者信息

Constantin Doru, Brotons Guillaume, Salditt Tim, Freyssingeas Eric, Madsen Anders

机构信息

Ecole Normale Supérieure de Lyon, Laboratoire de Physique, 46 Allée d'Italie, 69364 Lyon Cedex 07, France.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2006 Sep;74(3 Pt 1):031706. doi: 10.1103/PhysRevE.74.031706. Epub 2006 Sep 15.

Abstract

Using x-ray photon correlation spectroscopy, we studied the layer fluctuations in the lamellar phase of an ionic lyotropic system. We measured the relaxation rate of in-plane (undulation) fluctuations as a function of the wave vector. Static and dynamic results obtained during the same experiment were combined to yield the values of both elastic constants of the lamellar phase (compression and bending moduli) as well as that of the sliding viscosity. The results are in very good agreement with dynamic light-scattering data, validating the use of the technique in ordered phases.

摘要

我们使用X射线光子相关光谱法研究了离子型溶致体系层状相中的层波动。我们测量了面内(起伏)波动的弛豫速率作为波矢的函数。在同一实验中获得的静态和动态结果相结合,得出了层状相的两个弹性常数(压缩模量和弯曲模量)以及滑动粘度的值。结果与动态光散射数据非常吻合,验证了该技术在有序相中的应用。

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