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致密化对玻璃振动状态密度的影响。

Effect of densification on the density of vibrational states of glasses.

作者信息

Monaco A, Chumakov A I, Monaco G, Crichton W A, Meyer A, Comez L, Fioretto D, Korecki J, Rüffer R

机构信息

European Synchrotron Radiation Facility, BP 220, F-38043 Grenoble, France.

出版信息

Phys Rev Lett. 2006 Sep 29;97(13):135501. doi: 10.1103/PhysRevLett.97.135501. Epub 2006 Sep 25.

Abstract

We studied the effect of densification on the vibrational dynamics of a Na(2)FeSi(3)O(8) glass. The density of vibrational states (DOS) has been measured using nuclear inelastic scattering. The corresponding changes in the microscopic, intermediate-range, and macroscopic properties have also been investigated. The results reveal that, in the absence of local structure transformations, the Debye level and the glass-specific excess of vibrational states above it have the same dependence on density, and the evolution of the DOS is fully described by the transformation of the elastic medium.

摘要

我们研究了致密化对Na₂FeSi₃O₈玻璃振动动力学的影响。使用核非弹性散射测量了振动态密度(DOS)。还研究了微观、中程和宏观性质的相应变化。结果表明,在没有局部结构转变的情况下,德拜能级及其上方玻璃特有的振动态过量对密度具有相同的依赖性,并且DOS的演化完全由弹性介质的转变来描述。

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