Monaco A, Chumakov A I, Monaco G, Crichton W A, Meyer A, Comez L, Fioretto D, Korecki J, Rüffer R
European Synchrotron Radiation Facility, BP 220, F-38043 Grenoble, France.
Phys Rev Lett. 2006 Sep 29;97(13):135501. doi: 10.1103/PhysRevLett.97.135501. Epub 2006 Sep 25.
We studied the effect of densification on the vibrational dynamics of a Na(2)FeSi(3)O(8) glass. The density of vibrational states (DOS) has been measured using nuclear inelastic scattering. The corresponding changes in the microscopic, intermediate-range, and macroscopic properties have also been investigated. The results reveal that, in the absence of local structure transformations, the Debye level and the glass-specific excess of vibrational states above it have the same dependence on density, and the evolution of the DOS is fully described by the transformation of the elastic medium.
我们研究了致密化对Na₂FeSi₃O₈玻璃振动动力学的影响。使用核非弹性散射测量了振动态密度(DOS)。还研究了微观、中程和宏观性质的相应变化。结果表明,在没有局部结构转变的情况下,德拜能级及其上方玻璃特有的振动态过量对密度具有相同的依赖性,并且DOS的演化完全由弹性介质的转变来描述。