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二维非晶态固体中振动模式的实验研究。

Experimental studies of vibrational modes in a two-dimensional amorphous solid.

作者信息

Zhang Ling, Zheng Jie, Wang Yinqiao, Zhang Lei, Jin Zhaohui, Hong Liang, Wang Yujie, Zhang Jie

机构信息

School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai, 200240, China.

Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai, 200240, China.

出版信息

Nat Commun. 2017 Jul 10;8(1):67. doi: 10.1038/s41467-017-00106-5.

DOI:10.1038/s41467-017-00106-5
PMID:28694525
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5503991/
Abstract

The boson peak, which represents an excess of vibrational states compared to Debye's prediction at low frequencies, has been studied extensively, and yet, its nature remains controversial. In this study, we focus on understanding the nature of the boson peak based on the spatial heterogeneity of modulus fluctuations using a simple model system of a highly jammed two-dimensional granular material. Despite the simplicity of our system, we find that the boson peak in our two-dimensional system shows a shape very similar to that of three-dimensional molecular glasses when approaching their boson peak frequencies. Our finding indicates a strong connection between the boson peak and the spatial heterogeneity of shear modulus fluctuations.The low-frequency collective vibrational modes, known as the boson peak, characterize many glasses at low temperature, yet its origin remains elusive. Zhang et al. show a correlation between the boson peak and the spatial heterogeneity of shear modulus fluctuation in a two-dimensional granular system.

摘要

玻色子峰代表了在低频下与德拜预测相比振动状态的过剩,已经得到了广泛研究,然而其本质仍然存在争议。在本研究中,我们使用高度堵塞的二维颗粒材料的简单模型系统,基于模量涨落的空间异质性来专注于理解玻色子峰的本质。尽管我们的系统很简单,但我们发现二维系统中的玻色子峰在接近其玻色子峰频率时呈现出与三维分子玻璃非常相似的形状。我们的发现表明玻色子峰与剪切模量涨落的空间异质性之间存在紧密联系。低频集体振动模式,即所谓的玻色子峰,在低温下表征了许多玻璃,但其起源仍然难以捉摸。张等人展示了二维颗粒系统中玻色子峰与剪切模量涨落的空间异质性之间的相关性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/8997593dc670/41467_2017_106_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/c50df7292712/41467_2017_106_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/126ac69a041d/41467_2017_106_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/9cee59b182db/41467_2017_106_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/aa2d2fe651e5/41467_2017_106_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/77d2eb0097cc/41467_2017_106_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/8997593dc670/41467_2017_106_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/c50df7292712/41467_2017_106_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/126ac69a041d/41467_2017_106_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/9cee59b182db/41467_2017_106_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/aa2d2fe651e5/41467_2017_106_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/77d2eb0097cc/41467_2017_106_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/14e0/5503991/8997593dc670/41467_2017_106_Fig6_HTML.jpg

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本文引用的文献

1
Memory Effect Manifested by a Boson Peak in Metallic Glass.金属玻璃中玻色子峰所表现出的记忆效应。
Phys Rev Lett. 2016 Apr 29;116(17):175901. doi: 10.1103/PhysRevLett.116.175901. Epub 2016 Apr 27.
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Spatial Distributions of Local Elastic Moduli Near the Jamming Transition.近堵塞转变处局部弹性模量的空间分布
Phys Rev Lett. 2016 Feb 12;116(6):068302. doi: 10.1103/PhysRevLett.116.068302. Epub 2016 Feb 10.
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Probing the Role of Mobility in the Collective Motion of Nonequilibrium Systems.探究流动性在非平衡系统集体运动中的作用。
Phys Rev Lett. 2016 Jan 29;116(4):048302. doi: 10.1103/PhysRevLett.116.048302.
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Strain fluctuations and elastic moduli in disordered solids.无序固体中的应变涨落与弹性模量
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Disordered solids without well-defined transverse phonons: the nature of hard-sphere glasses.无序固体中没有明确的横向声子:硬球玻璃的本质。
Phys Rev Lett. 2015 Jan 23;114(3):035502. doi: 10.1103/PhysRevLett.114.035502.
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Effects of coordination and pressure on sound attenuation, boson peak and elasticity in amorphous solids.配位和压力对非晶态固体中声衰减、玻色子峰及弹性的影响。
Soft Matter. 2014 Aug 14;10(30):5628-44. doi: 10.1039/c4sm00561a.
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Phonon dispersion and elastic moduli of two-dimensional disordered colloidal packings of soft particles with frictional interactions.具有摩擦相互作用的软颗粒二维无序胶体填料的声子色散和弹性模量
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Heterogeneous shear elasticity of glasses: the origin of the boson peak.玻璃的非均匀剪切弹性:玻色峰的起源。
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