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表面活性剂改性天然沸石去除苯酚和4-氯苯酚

Removal of phenol and 4-chlorophenol by surfactant-modified natural zeolite.

作者信息

Kuleyin Ayşe

机构信息

Environmental Engineering Department, Ondokuzmayis University, 55139 Samsun, Turkey.

出版信息

J Hazard Mater. 2007 Jun 1;144(1-2):307-15. doi: 10.1016/j.jhazmat.2006.10.036. Epub 2006 Oct 15.

DOI:10.1016/j.jhazmat.2006.10.036
PMID:17112660
Abstract

In this study the adsorption characteristics of phenol and 4-chlorophenol by surfactant-modified zeolite was investigated. Batch studies were performed to evaluate the effects of various experimental parameters such as contact time, adsorbent dose, initial concentration, and temperature on the removal of phenol and 4-chlorophenol. The sorption kinetics was tested for intraparticle diffusion, Elovich, and pseudo-second order reaction and rate constants of kinetic models were calculated. Equilibrium isotherms for the adsorption of phenol were analyzed by Freundlich, Langmuir, and Tempkin isotherm models. Freundlich isotherm was found to best represent the data for phenol and 4-chlorophenol adsorption.

摘要

本研究考察了表面活性剂改性沸石对苯酚和4-氯苯酚的吸附特性。进行了批量研究，以评估接触时间、吸附剂剂量、初始浓度和温度等各种实验参数对苯酚和4-氯苯酚去除效果的影响。测试了颗粒内扩散、埃洛维奇方程和伪二级反应的吸附动力学，并计算了动力学模型的速率常数。采用弗伦德里希、朗缪尔和坦普金等温线模型分析了苯酚吸附的平衡等温线。结果发现，弗伦德里希等温线最能代表苯酚和4-氯苯酚吸附的数据。

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