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俄罗斯亚洲北极地区两个地下核爆炸地点周围的地表污染及土壤中137Cs的垂直分布

Surface ground contamination and soil vertical distribution of 137Cs around two underground nuclear explosion sites in the Asian Arctic, Russia.

作者信息

Ramzaev Valery, Mishine Arkady, Golikov Vladislav, Brown Justin Emrys, Strand Per

机构信息

St.-Petersburg Institute of Radiation Hygiene, Mira street 8, 197101, St.-Petersburg, Russia.

出版信息

J Environ Radioact. 2007;92(3):123-43. doi: 10.1016/j.jenvrad.2006.10.001. Epub 2006 Dec 5.

DOI:10.1016/j.jenvrad.2006.10.001
PMID:17156902
Abstract

Vertical distributions of 137Cs have been determined in vegetation-soil cores obtained from 30 different locations around two underground nuclear explosion sites--"Crystal" (event year - 1974) and "Kraton-3" (event year - 1978) in the Republic of Sakha (Yakutia), Russia. In 2001-2002, background levels of 137Cs surface contamination densities on control forest plots varied from 0.73 to 0.97 kBq m(-2) with an average of 0.84+/-0.10 kBq m(-2) and a median of 0.82 kBq m(-2). 137Cs ground contamination densities at the "Crystal" site ranged from 1.3 to 64 kBq m(-2); the activity gradually decreased with distance from the borehole. For "Kraton-3", residual surface contamination density of radiocaesium varied drastically from 1.7 to 6900 kBq m(-2); maximal 137Cs depositions were found at a "decontaminated" plot. At all forest plots, radiocaesium activity decreased throughout the whole vertical soil profile. Vertical distributions of 137Cs in soil for the majority of the plots sampled (n=18) can be described using a simple exponential function. Despite the fact that more than 20 years have passed since the main fallout events, more than 80% of the total deposited activity was found in the first 5 cm of the vegetation-soil cores from most of the forested landscapes. The low annual temperatures, clay-rich soil type with neutral pH, and presence of thick lichen-moss carpet are the factors which may hinder 137Cs transport down the soil profile.

摘要

已测定了从俄罗斯萨哈(雅库特)共和国两个地下核爆炸地点——“水晶”(爆炸年份 - 1974年)和“克拉通 - 3”(爆炸年份 - 1978年)周围30个不同地点采集的植被 - 土壤岩芯中¹³⁷Cs的垂直分布情况。在2001 - 2002年期间,对照森林地块上¹³⁷Cs表面污染密度的背景水平在0.73至0.97 kBq m⁻²之间变化,平均为0.84±0.10 kBq m⁻²,中位数为0.82 kBq m⁻²。“水晶”地点的¹³⁷Cs地面污染密度在1.3至64 kBq m⁻²之间;其活度随离钻孔距离的增加而逐渐降低。对于“克拉通 - 3”,放射性铯的残留表面污染密度变化极大,从1.7至6900 kBq m⁻²不等;在一个“已去污”地块发现了最大的¹³⁷Cs沉积量。在所有森林地块中,放射性铯活度在整个土壤垂直剖面中均降低。对于大多数采样地块(n = 18),土壤中¹³⁷Cs的垂直分布可用一个简单的指数函数来描述。尽管自主要沉降事件发生以来已过去20多年,但在大多数森林景观的植被 - 土壤岩芯的前5厘米中发现了超过80%的总沉积活度。年平均气温较低、土壤类型为富含黏土且pH值呈中性以及存在厚厚的地衣 - 苔藓层,这些因素可能会阻碍¹³⁷Cs在土壤剖面中的向下迁移。

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