Monn James A, Massey Steven M, Valli Matthew J, Henry Steven S, Stephenson Gregory A, Bures Mark, Hérin Marc, Catlow John, Giera Deborah, Wright Rebecca A, Johnson Bryan G, Andis Sherri L, Kingston Ann, Schoepp Darryle D
Neuroscience Research Division, Eli Lilly and Company, Indianapolis, Indiana 46285, USA.
J Med Chem. 2007 Jan 25;50(2):233-40. doi: 10.1021/jm060917u.
(-)-4-Amino-2-thiabicyclo-[3.1.0]hexane-4,6-dicarboxylate (LY389795, (-)-3) is a highly potent and selective agonist of metabotropic glutamate receptors 2 (mGlu2) and 3 (mGlu3). As part of our ongoing research program, we have prepared S-oxidized variants of (-)-3, compounds (-)-10, (+)-11 (LY404040), and (-)-12 (LY404039). Each of these chiral heterobicyclic amino acids displaced specific binding of the mGlu2/3 receptor antagonist 3H-2S-2-amino-2-(1S,2S-2-carboxycycloprop-1-yl)-3-(xanth-9-yl)propanoic acid (3H-LY341495) from membranes expressing recombinant human mGlu2 or mGlu3 and acted as potent agonists in cells expressing these receptor subtypes. Docking of the most potent of these derivatives, (+)-11, to mGlu2 revealed the possibility of an additional H-bond interaction between the sulfoxide oxygen of (+)-11 with tyrosine residue Y236. Pharmacokinetic analysis of mGlu active enantiomers (+)-11 and (-)-12 in rats showed each to be well absorbed following oral administration. Consistent with their mGlu2/3 agonist potency and pharmacokinetic properties, both (+)-11 and (-)-12 blocked phencyclidine-evoked ambulations in a dose-dependent manner, indicating their potential as nonclassical antipsychotic agents.
(-)-4-氨基-2-硫杂双环-[3.1.0]己烷-4,6-二羧酸酯(LY389795,(-)-3)是代谢型谷氨酸受体2(mGlu2)和3(mGlu3)的高效选择性激动剂。作为我们正在进行的研究项目的一部分,我们制备了(-)-3的S-氧化变体化合物(-)-10、(+)-11(LY404040)和(-)-12(LY404039)。这些手性杂环氨基酸中的每一种都能从表达重组人mGlu2或mGlu3的膜中取代mGlu2/3受体拮抗剂3H-2S-2-氨基-2-(1S,2S-2-羧基环丙-1-基)-3-(呫吨-9-基)丙酸(3H-LY341495)的特异性结合,并在表达这些受体亚型的细胞中作为强效激动剂发挥作用。这些衍生物中最有效的(+)-11与mGlu2对接显示,(+)-11的亚砜氧与酪氨酸残基Y236之间可能存在额外的氢键相互作用。对大鼠体内mGlu活性对映体(+)-11和(-)-12的药代动力学分析表明,口服给药后它们的吸收都很好。与它们的mGlu2/3激动剂效力和药代动力学性质一致,(+)-11和(-)-12均以剂量依赖性方式阻断苯环利定诱发走动,表明它们作为非经典抗精神病药物的潜力。