Muench Stephen P, Prigge Sean T, McLeod Rima, Rafferty John B, Kirisits Michael J, Roberts Craig W, Mui Ernest J, Rice David W
The Krebs Institute for Biomolecular Research, Department of Molecular Biology and Biotechnology, University of Sheffield, Firth Court, Western Bank, Sheffield S10 2TN, England.
Acta Crystallogr D Biol Crystallogr. 2007 Mar;63(Pt 3):328-38. doi: 10.1107/S0907444906053625. Epub 2007 Feb 21.
Recent studies have demonstrated that submicromolar concentrations of the biocide triclosan arrest the growth of the apicomplexan parasites Plasmodium falciparum and Toxoplasma gondii and inhibit the activity of the apicomplexan enoyl acyl carrier protein reductase (ENR). The crystal structures of T. gondii and P. falciparum ENR in complex with NAD(+) and triclosan and of T. gondii ENR in an apo form have been solved to 2.6, 2.2 and 2.8 A, respectively. The structures of T. gondii ENR have revealed that, as in its bacterial and plant homologues, a loop region which flanks the active site becomes ordered upon inhibitor binding, resulting in the slow tight binding of triclosan. In addition, the T. gondii ENR-triclosan complex reveals the folding of a hydrophilic insert common to the apicomplexan family that flanks the substrate-binding domain and is disordered in all other reported apicomplexan ENR structures. Structural comparison of the apicomplexan ENR structures with their bacterial and plant counterparts has revealed that although the active sites of the parasite enzymes are broadly similar to those of their bacterial counterparts, there are a number of important differences within the drug-binding pocket that reduce the packing interactions formed with several inhibitors in the apicomplexan ENR enzymes. Together with other significant structural differences, this provides a possible explanation of the lower affinity of the parasite ENR enzyme family for aminopyridine-based inhibitors, suggesting that an effective antiparasitic agent may well be distinct from equivalent antimicrobials.
最近的研究表明,亚微摩尔浓度的杀菌剂三氯生可抑制顶复门寄生虫恶性疟原虫和刚地弓形虫的生长,并抑制顶复门烯酰酰基载体蛋白还原酶(ENR)的活性。已分别解析出与NAD(+)和三氯生结合的刚地弓形虫和恶性疟原虫ENR的晶体结构,以及无配体形式的刚地弓形虫ENR的晶体结构,分辨率分别为2.6埃、2.2埃和2.8埃。刚地弓形虫ENR的结构表明,与其细菌和植物同源物一样,活性位点两侧的一个环区域在抑制剂结合后变得有序,导致三氯生的缓慢紧密结合。此外,刚地弓形虫ENR-三氯生复合物揭示了顶复门家族共有的一个亲水性插入片段的折叠情况,该片段位于底物结合结构域的两侧,在所有其他已报道的顶复门ENR结构中是无序的。将顶复门ENR结构与其细菌和植物对应物进行结构比较发现,尽管寄生虫酶的活性位点与细菌对应物大致相似,但药物结合口袋内存在一些重要差异,这些差异减少了与顶复门ENR酶中几种抑制剂形成的堆积相互作用。连同其他显著的结构差异,这可能解释了寄生虫ENR酶家族对基于氨基吡啶的抑制剂亲和力较低的原因,表明有效的抗寄生虫药物可能与等效的抗菌药物截然不同。