Hess C, Elhaes H, Waske A, Büchner B, Sekar C, Krabbes G, Heidrich-Meisner F, Brenig W
Leibniz-Institute for Solid State and Materials Research, IFW-Dresden, 01171 Dresden, Germany.
Phys Rev Lett. 2007 Jan 12;98(2):027201. doi: 10.1103/PhysRevLett.98.027201. Epub 2007 Jan 10.
We present experimental results for the thermal conductivity kappa of the pseudo-two-leg ladder material CaCu2O3. The strong buckling of the ladder rungs renders this material a good approximation to a S=1/2 Heisenberg chain. Despite a strong suppression of the thermal conductivity of this material in all crystal directions due to inherent disorder, we find a dominant magnetic contribution kappa mag along the chain direction. kappa mag is linear in temperature, resembling the low-temperature limit of the thermal Drude weight D th of the S=1/2 Heisenberg chain. The comparison of kappamag and Dth yields a magnetic mean-free path of l mag approximately 22+/-5 A, in good agreement with magnetic measurements.