Lebreton L, Zimbal A, Thomas D
Institut de radioprotection et de sûreté nucléaire (IRSN), Saint-Paul-Lez-Durance, France.
Radiat Prot Dosimetry. 2007;126(1-4):3-7. doi: 10.1093/rpd/ncm003. Epub 2007 May 17.
(241)Am-Be(alpha,n) neutron sources provide one of the most commonly used neutron fields for routine calibration of neutron sensitive devices. The neutron energy distribution of the IRSN standard (241)Am-Be source was measured in the energy region above 1.65 MeV using a BC501A proton-recoil liquid scintillator. The experimental data were compared to the ISO-recommended neutron energy distribution for an (241)Am-Be source. Some differences in shape were observed, with large variations mainly within the energy interval 3-6 MeV and around 8 MeV. Within the framework of a collaboration between three national metrological institutes (PTB, Germany; NPL, UK and LNE-IRSN, France), the neutron energy distributions of (241)Am-Be sources at each laboratory have been compared. The IRSN-BC501A proton-recoil scintillator was used to measure all the sources. The results show different energy distributions a priori influenced by the origin of the source, i.e. the manufacturing process. The maximum deviation observed for the integral dose equivalent, in the measured BC501A energy range, is within the 4% uncertainty recommended by ISO standard 8529-2 to allow for variations of the neutron spectrum among different (241)Am-Be sources. However, knowledge of the energy distribution of an (241)Am-Be source provides a way to reduce the uncertainty in the dose equivalent rate delivered by such a source.
(241)镅铍(α,n)中子源是用于中子敏感设备常规校准的最常用中子场之一。使用BC501A质子反冲液体闪烁体在1.65 MeV以上的能量区域测量了法国国家辐射防护与核能安全研究所(IRSN)标准(241)镅铍源的中子能量分布。将实验数据与ISO推荐的(241)镅铍源中子能量分布进行了比较。观察到形状上存在一些差异,主要在3 - 6 MeV能量区间和8 MeV左右有较大变化。在三个国家计量机构(德国物理技术研究院(PTB)、英国国家物理实验室(NPL)和法国国家计量院 - IRSN)合作的框架内,对每个实验室的(241)镅铍源的中子能量分布进行了比较。所有源均使用IRSN - BC501A质子反冲闪烁体进行测量。结果表明,能量分布因源的产地即制造工艺而存在先验差异。在测量的BC501A能量范围内,观察到的积分剂量当量的最大偏差在ISO标准8529 - 2推荐的4%不确定度范围内,该不确定度用于考虑不同(241)镅铍源之间中子能谱的变化。然而,了解(241)镅铍源的能量分布提供了一种降低此类源所提供剂量当量率不确定度的方法。