Science. 1990 Sep 21;249(4975):1382-6. doi: 10.1126/science.249.4975.1382.
A new model has been constructed for calculating the level of atmospheric CO(2) during the past 570 million years. A series of successive steady states for CO(2) is used in order to calculate CO(2) level from a feedback function for the weathering of silicate minerals. Processes considered are: sedimentary burial of organic matter and carbonates; continental weathering of silicates, carbonates, and organic matter; and volcanic and metamorphic degassing of CO(2). Sediment burial rates are calculated with the use of an isotope mass-balance model and carbon isotopic data on ancient seawater. Weathering rates are calculated from estimates of past changes in continental land area, mean elevation, and river runoff combined with estimates of the effects of the evolution of vascular land plants. Past degassing rates are estimated from changes in the rate of generation of sea floor and the shift of carbonate deposition from platforms to the deep sea. The model results indicate that CO(2) levels were high during the Mesozoic and early Paleozoic and low during the Permo-Carboniferous and late Cenozoic. These results correspond to independently deduced Phanerozoic paleoclimates and support the notion that the atmospheric CO(2) greenhouse mechanism is a major control on climate over very long time scales.
已经构建了一个新模型来计算过去 5.7 亿年来大气中 CO2 的水平。为了从硅酸盐矿物风化的反馈函数中计算 CO2 的水平,使用了一系列连续的稳定状态。所考虑的过程包括:有机物和碳酸盐的沉积埋藏;硅酸盐、碳酸盐和有机物的大陆风化;以及火山和变质作用下 CO2 的排放。利用同位素质量平衡模型和古代海水的碳同位素数据来计算沉积物埋藏速率。风化速率是根据过去大陆面积、平均海拔和河流径流量变化的估计值以及维管束陆地植物进化影响的估计值计算得出的。过去的脱气速率是根据海底生成速率的变化和碳酸盐沉积从台地向深海转移的变化来估计的。模型结果表明,CO2 水平在中生代和早古生代较高,在石炭纪-二叠纪和晚新生代较低。这些结果与独立推断的显生宙古气候相对应,并支持大气 CO2 温室机制是对超长时间尺度气候的主要控制的观点。